Shape coexistence in the neutron-deficient even-even Hg182-188 isotopes studied via Coulomb excitation

Coulomb-excitation experiments to study electromagnetic properties of radioactive even-even Hg isotopes were performed with 2.85  MeV/nucleon mercury beams from REX-ISOLDE. Magnitudes and relative signs of the reduced E2 matrix elements that couple the ground state and low-lying excited states in Hg182-188 were extracted. Information on the deformation of the ground and the first excited 0+ states was deduced using the quadrupole sum rules approach. Results show that the ground state is slightly deformed and of oblate nature, while a larger deformation for the excited 0+ state was noted in Hg182,184. The results are compared to beyond mean field and interacting-boson based models and interp…

Structure of the As, Ge, Ga nuclei

Abstract The level structures of the N = 50 83As, 82Ge, and 81Ga isotones have been investigated by means of multi-nucleon transfer reactions. A first experiment was performed with the CLARA–PRISMA setup to identify these nuclei. A second experiment was carried out with the GASP array in order to deduce the γ-ray coincidence information. The results obtained on the high-spin states of such nuclei are used to test the stability of the N = 50 shell closure in the region of 78Ni ( Z = 28 ). The comparison of the experimental level schemes with the shell-model calculations yields an N = 50 energy gap value of 4.7(3) MeV at Z = 28 . This value, in a good agreement with the prediction of the fini…

α -decay spectroscopy of the N=130 isotones Ra218 and Th220 : Mitigation of α -particle energy summing with implanted nuclei

© 2019 American Physical Society. An analysis technique has been developed in order to mitigate energy summing due to sequential short-lived α decays from nuclei implanted into a silicon detector. Using this technique, α-decay spectroscopy of the N=130 isotones Ra218 (Z=88) and Th220 (Z=90) has been performed. The energies of the α particles emitted in the Ra218→Rn214 and Th220→Ra216 ground-state-to-ground-state decays have been measured to be 8381(4) keV and 8818(13) keV, respectively. The half-lives of the ground states of Ra218 and Th220 have been measured to be 25.99(10) μs and 10.4(4) μs, respectively. The half-lives of the ground states of the α-decay daughters, Rn214 and Ra216, have …

γ-ray spectroscopy of neutron-deficientTe110. II. High-spin smooth-terminating structures

High-spin states have been populated in Te-110(52) via Ni-58(Ni-58,alpha 2p gamma) reactions at 240 and 250 MeV. The Gammasphere gamma-ray spectrometer was used in conjunction with the Microball charged-particle detector. The high-spin (I>30) collective level scheme of Te-110, up to similar to 45h, is discussed in this paper. Four new decoupled (Delta I=2) high-spin structures have been observed for the first time, together with two strongly coupled (Delta I=1) bands. These bands all show the characteristics of smooth band termination, and are discussed within the framework of the cranked Nilsson-Strutinsky approach.

Isomers and high-spin structures in the N=81 isotones Xe135 and Ba137

The high-spin structures of the N = 81 isotones 135Xe and 137Ba are investigated after multinucleontransfer (MNT) and fusion-evaporation reactions. Both nuclei are populated in (i) 136Xe+238U and (ii) 136Xe+208Pb MNT reactions employing the high-resolution Advanced Gamma Tracking Array (AGATA) coupled to the magnetic spectrometer PRISMA, (iii), in the 136Xe+198Pt MNT reaction employing the -ray array GAMMASPHERE in combination with the gas detector array Chico, and (iv) via a 11B+130Te fusion-evaporation reaction. The high-spin level schemes of 135Xe and 137Ba are considerably extended to higher energies. The 2058-keV (19=2 ) state in 135Xe is identified as an isomer, completing the systema…

Identification of the Jπ = 1− state in 218Ra populated via α decay of 222Th

The α decay of 222Th populating the low-lying J π = 3− state, and also a proposed 1− state, in 218Ra has been observed. The observations suggest an excitation energy of 853 keV for the 1− state, which is 60 keV above the 3− state. The hindrance factors of these α decays give a possible boundary to the region of ground-state octupole deformation in the light-actinide nuclei. The relative positions of the J π = 1− and 3− states suggest they are produced by an octupole-vibrational mechanism, as opposed to α clustering or rotations of a reflection-asymmetric octupole-deformed shape. peerReviewed

A time-of-flight correction procedure for fast-timing data of recoils with varying implantation positions at a spectrometer focal plane

Abstract Fast-timing measurements at the focal plane of a separator can suffer from poor timing resolution. This is due to the variations in time-of-flight (ToF) for photons travelling to a given detector, which arise from the changes in the implantation positions of the recoil nuclei emitting the γ rays of interest. In order to minimise these effects on timing measurements, a procedure is presented that improves fast-timing data by performing ToF corrections on an event-by-event basis. This method was used to correct data collected with an array of eight LaBr 3 detectors, which detected γ rays from spatially distributed 138Gd recoil-implants at the focal plane of the Recoil-Ion-Transport-U…

Evidence for Magnetic Rotation in the Light Tin Region

Lifetimes have been measured for three M1 bands in light Sn/Cd nuclei using the DSAM technique. B(M1) values deduced from these measurements show a rapid decrease with increasing spin for a given configuration. The results have been compared with both Tilted axis cranking and semi-empirical model calculations. These suggest that the shears mechanism is present in this mass region, and that the band in 106Sn appears to be the first example of almost pure magnetic rotation.

Fine structure in the α decay of 156Lu and 158Ta

Fine structure in the α decay of high-spin states in 156Lu and 158Ta has been identified by means of αγ - coincidence analysis. One new α decay from 156Lu and two from 158Ta were identified, one of which was found to populate a previously unknown state in 154Lu. The hindrance-factor systematics from all four odd-odd, N = 85 nuclei with known α-decaying, πh11/2 coupled states were reviewed and are discussed. These proved consistent with the previously assigned (πh11/2νh9/2 )10+ configuration of the α-decaying state in 156Lu, which differs from the (πh11/2ν f7/2 )9+ assignments in the other three nuclei. peerReviewed

Neutron configurations in 113Pd

Excited states in 113Pd, populated in β− decay of 113Rh and in spontaneous fission of 248Cm and 252Cf, have been studied by means of γ spectroscopy at the IGISOL facility of Jyvaskylä University and using large arrays of Ge detectors (Eurogam2 and Gammasphere, respectively). The position of the 11/2− yrast excitation in 113Pd, proposed recently at 166.1 keV by other authors, has been corrected to 98.9 keV. The decay of this level has been discussed to explain the observed transition intensities. The 7/2− member of the yrast, unique-parity configuration has been identified at 84.9 keV and a band on top of this level proposed. On top of the 1/2+, first excited state a band has been built and …

Excited states in Ra217 populated in the α decay of Th221

Fine structure in the α decay of Th90221, populating excited states in Ra88217, was studied using αγ-coincidence spectroscopy. Two α-decay branches from Th221 have been newly observed, with Eα(keV)[bα(%)]=7951(8)[0.14(3)] and 8247(3)[1.51(12)], together with three previously known branches. Also, two new states in Ra217 were identified at E = 177 and 227 keV. The ground-state configurations of the odd-A, N = 131 transitional isotones above Pb208 are interpreted from their α-decay fine structure systematics and considered in terms of predictions using spherical shell and reflection-asymmetric models.

A charge plunger device to measure the lifetimes of excited nuclear states where transitions are dominated by internal conversion

Abstract A charge plunger device has been commissioned based on the DPUNS plunger (Taylor et al., 2013) using the in-flight mass separator MARA at the University of Jyvaskyla. The 152 Sm (32 S ,4 n )180 Pt reaction was used to populate excited states in 180 Pt . A lifetime measurement of the 2 1 + state was performed by applying the charge plunger technique, which relies on the detection of the charge state-distribution of recoils rather than the detection of the emitted γ rays. This state was a good candidate to test the charge plunger technique as it has a known lifetime and depopulates through a converted transition that competes strongly with γ -ray emission. The lifetime of the 2 1 + s…

Direct observation of theBa114→Xe110→Te106→Sn102tripleα-decay chain using position and time correlations

The triple $\ensuremath{\alpha}$-decay chain $^{114}\mathrm{Ba}\ensuremath{\rightarrow}^{110}\mathrm{Xe}\ensuremath{\rightarrow}^{106}\mathrm{Te}\ensuremath{\rightarrow}^{102}\mathrm{Sn}$ has been directly observed for the first time, following the $^{58}\mathrm{Ni}(^{58}\mathrm{Ni},2n)$ reaction. Implantation of $^{114}\mathrm{Ba}$ nuclei into a double-sided silicon-strip detector has allowed their $\ensuremath{\alpha}$ decays to be correlated in position and time with the $\ensuremath{\alpha}$ decays of the daughter $(^{110}\mathrm{Xe})$ and granddaughter $(^{106}\mathrm{Te})$ nuclei. In total, 17 events have been assigned to the $^{114}\mathrm{Ba}\ensuremath{\rightarrow}^{110}\mathrm{Xe}…

Decay of a 19(-) isomeric state in Lu-156

A multiparticle spin-trap isomeric state having a half-life of 179(4) ns and lying 2601 keV above the yrast 10(+) state in Lu-156 has been discovered. The Lu-156 nuclei were produced by bombarding isotopically enriched Cd-106 targets with beams of Ni-58 ions, separated in flight using the gas-filled separator RITU and their decays were measured using the GREAT spectrometer. Analysis of the main decay path that populates yrast states observed previously suggests a spin-parity assignment of 19(-) for the isomeric state, which is consistent with isomeric states identified in the N = 85 isotones. Comparison with other decay paths in Lu-156 indicates that the [pi h(11/)(2)(-1) circle times nu h(…

Evidence for Shears Bands in108Cd

High-spin states were populated in ${}^{108}\mathrm{Cd}$ using the ${}^{96}\mathrm{Zr}{(}^{16}\mathrm{O},4n)$ reaction at a beam energy of 72 MeV. Two magnetic dipole bands have been observed, both of which contain weak $E2$ crossover transitions. Lifetimes for the stronger of the two bands were measured via the Doppler shift attenuation method. The configuration assignment for this band has been determined from comparison with tilted axis cranking model calculations to be $\ensuremath{\pi}[{g}_{9/2}^{\ensuremath{-}3}{g}_{7/2}]\ensuremath{\bigotimes}\ensuremath{\nu}[{h}_{11/2}{(g}_{7/2}{d}_{5/2}{)}^{1}]$ and $\ensuremath{\pi}[{g}_{9/2}^{\ensuremath{-}3}{g}_{7/2}]\ensuremath{\bigotimes}\ensu…

Identification of excited states in119Ba

Excited states have been identified in the very neutron-deficient ${}^{119}\mathrm{Ba}$ nucleus. Two bands have been observed, which are likely to be based on ${h}_{11/2}$ and ${(g}_{7/2}{d}_{5/2})$ neutron orbitals. Despite this being the first observation of excited states in ${}^{119}\mathrm{Ba},$ the bands extend to $(75/2)\ensuremath{\Elzxh}$ and $(79/2)\ensuremath{\Elzxh},$ respectively. The bands have been assigned to ${}^{119}\mathrm{Ba}$ using gamma-recoil and gamma--x-ray coincidences. Several quasiparticle alignments have been identified, involving neutron ${(h}_{11/2}{)}^{2}$ and proton ${(h}_{11/2}{)}^{2}$ aligned configurations. Furthermore, the bands show features which are r…

Spectroscopic study of228-234Th nuclei using multi-nucleon transfer reactions

Light-actinide nuclei in the octupole deformed region have been populated using multi-nucleon transfer from Th. The energy level schemes of several thorium isotopes with A = 228-234 have been extended up to and negative parity states have been observed for the first time in Th. A systematic study of the difference in alignment between the positive- and negative-parity bands in thorium nuclei in this mass region shows that Th behave like octupole vibrators, in contrast with Th, which are octupole-deformed in character. An intrinsic electric dipole moment has been measured for the first time in Th. The small value obtained is consistent with the vibrational description of this nucleus.

Direct observation of the Ba 114 → Xe 110 → Te 106 → Sn 102 triple α -decay chain using position and time correlations

The triple α-decay chain 114Ba → 110Xe → 106Te → 102Sn has been directly observed for the first time, following the 58Ni(58Ni ,2n) reaction. Implantation of 114Ba nuclei into a double-sided silicon-strip detector has allowed their α decays to be correlated in position and time with the α decays of the daughter (110Xe) and granddaughter (106Te) nuclei. In total, 17 events have been assigned to the 114Ba → 110Xe → 106Te → 102Sn triple α-decay chain. The energy of the 114Ba α decay has been measured to be Eα = 3480(20) keV, which is 70 keV higher than the previously measured value, and the half-life of 114Ba has been measured with improved accuracy, to be 380+190 −110 ms. A revised Q12C value …

Decay of a 19− isomeric state in 156Lu

A multiparticle spin-trap isomeric state having a half-life of 179(4) ns and lying 2601 keV above the yrast 10 + state in 156 Lu has been discovered. The 156 Lu nuclei were produced by bombarding isotopically enriched 106 Cd targets with beams of 58 Ni ions, separated in flight using the gas-filled separator RITU and their decays were measured using the GREAT spectrometer. Analysis of the main decay path that populates yrast states observed previously suggests a spin-parity assignment of 19 − for the isomeric state, which is consistent with isomeric states identified in the N = 85 isotones. Comparison with other decay paths in 156 Lu indicates that the [ π h − 1 11 / 2 ⊗ ν h 9 / 2 ] 10 + st…

Coulomb excitation of Rn-222

The nature of quadrupole and octupole collectivity in 222Rn was investigated by determining the electric-quadrupole (E2) and octupole (E3) matrix elements using subbarrier, multistep Coulomb excitation. The radioactive 222Rn beam, accelerated to 4.23 MeV/u, was provided by the HIE-ISOLDE facility at CERN. Data were collected in the Miniball γ-ray spectrometer following the bombardment of two targets, 120Sn and 60Ni. Transition E2 matrix elements within the ground-state and octupole bands were measured up to 10ℏ and the results were consistent with a constant intrinsic electric-quadrupole moment, 518(11)efm2. The values of the intrinsic electric-octupole moment for the 0+→3− and 2+→5− transi…

Study of medium-spin states of neutron-rich 87, 89, 91Rb isotopes

International audience; Excited states of the rubidium isotopes$_{37}^{87, 89, 91}$Rb have been studied at the INFN Legnaro National Laboratory. Measurements of the $\gamma$ -ray decay of fragments produced in binary grazing reactions resulting from the interaction of a beam of 530 MeV$^{96}$Zr ions with a$^{124}$Sn target have been complemented by studies of the $\gamma$ -ray decay of fission fragments produced in the interaction of a beam of 230 MeV$^{36}$S ions with a thick$^{176}$Yb target. The structure of the yrast states of$_{37}^{87, 89, 91}$Rb has been discussed within the context of spherical shell-model and cranked Nilsson-Strutinsky calculations.

Collectivity in the light radon nuclei measured directly via Coulomb excitation

Background: Shape coexistence in heavy nuclei poses a strong challenge to state-of-the-art nuclear models, where several competing shape minima are found close to the ground state. A classic region for investigating this phenomenon is in the region around Z=82 and the neutron midshell at N=104. Purpose: Evidence for shape coexistence has been inferred from α-decay measurements, laser spectroscopy, and in-beam measurements. While the latter allow the pattern of excited states and rotational band structures to be mapped out, a detailed understanding of shape coexistence can only come from measurements of electromagnetic matrix elements. Method: Secondary, radioactive ion beams of Rn202 and Rn…

Lifetime measurements of lowest states in the π g7/2 ⊗ νh11/2 rotational band in 112I

A differential-plunger device was used to measure the lifetimes of the lowest states in the πg7/2 ⊗ νh11/2 rotational band in doubly odd 112I with the 58Ni(58Ni, 3pn) reaction. A differential decay curve method was performed using the fully shifted and degraded γ -ray intensity measurements as a function of target-to-degrader distance. The lifetimes of the lowest three states in the πg7/2 ⊗ νh11/2 band in 112I were measured to be 124(30), 130(25), and 6.5(5) ps, respectively. As the lifetimes of successive excited states in a rotational band are expected to decrease with increasing excitation energy, these measurements suggest that the order of the transitions in the established band in 112…

Lifetime measurements of yrast states in ¹⁷⁸ Pt using the charge plunger method with a recoil separator

Abstract Lifetime measurements in \(^{178}\)Pt with excited states de-exciting through \(\gamma\)-ray transitions and internal electron conversions have been performed. Ionic charges were selected by the in-flight mass separator MARA and measured at the focal plane in coincidence with the \(4^{+}_{1}→2^{+}_{1}\) 257 keV γ-ray transition detected using the JUROGAM 3 spectrometer. The resulting charge-state distributions were analysed using the differential decay curve method (DDCM) framework to obtain a lifetime value of 430(20) ps for the \(2^{+}_{1}\) state. This work builds on a method that combines the charge plunger technique with the DDCM analysis. As an alternative analysis, ions were…

Deformation of the proton emitter 113Cs from electromagnetic transition and proton-emission rates

The lifetime of the (11/2+) state in the band above the proton-emitting (3/2+) state in 113Cs has been measured to be τ = 24(6) ps from a recoil-decay-tagged differential-plunger experiment. The measured lifetime was used to deduce the deformation of the states using wave functions from a nonadiabatic quasiparticle model to independently calculate both proton-emission and electromagnetic γ -ray transition rates as a function of deformation. The only quadrupole deformation, which was able to reproduce the experimental excitation energies of the states, the electromagnetic decay rate of the (11/2+) state and the proton-emission rate of the (3/2+) state, was found to be β2 = 0.22(6). This defo…

High-spin structures in Xe132 and Xe133 and evidence for isomers along the N=79 isotones

Author(s): Vogt, A; Siciliano, M; Birkenbach, B; Reiter, P; Hadynska-Klȩk, K; Wheldon, C; Valiente-Dobon, JJ; Teruya, E; Yoshinaga, N; Arnswald, K; Bazzacco, D; Blazhev, A; Bracco, A; Bruyneel, B; Chakrawarthy, RS; Chapman, R; Cline, D; Corradi, L; Crespi, FCL; Cromaz, M; De Angelis, G; Eberth, J; Fallon, P; Farnea, E; Fioretto, E; Fransen, C; Freeman, SJ; Fu, B; Gadea, A; Gelletly, W; Giaz, A; Gorgen, A; Gottardo, A; Hayes, AB; Hess, H; Hetzenegger, R; Hirsch, R; Hua, H; John, PR; Jolie, J; Jungclaus, A; Karayonchev, V; Kaya, L; Korten, W; Lee, IY; Leoni, S; Liang, X; Lunardi, S; MacChiavelli, AO; Menegazzo, R; Mengoni, D; Michelagnoli, C; Mijatovic, T; Montagnoli, G; Montanari, D; Muller-…

Fine structure in the α decay of high-spin isomers in 155Lu and 156Hf

Fine structure in the α decay of high-spin isomers in 155Lu(25/2−) and 156Hf (8+) has been studied for the first time using αγ -coincidence analysis. Three new α decays from 155Lu(25/2−) and two from 156Hf (8+) have been identified, populating seniority s > 1 states in the N = 82 nuclei 151Tm and 152Yb, respectively. The reduced hindrance factors of the α decays support the previous configuration assignments of the populated states. This is the first observation of states with excitation energy greater than 1.5 MeV being populated following α decay in nuclei outside of the 208Pb region. peerReviewed

Decay of a 19− isomeric state in Lu156

A multiparticle spin-trap isomeric state having a half-life of 179(4) ns and lying 2601 keV above the yrast 10(+) state in Lu-156 has been discovered. The Lu-156 nuclei were produced by bombarding ...

Lifetime measurements of lowest states in the πg7/2⊗νh11/2 rotational band in I112

Single-neutron orbits near 78 Ni: Spectroscopy of theN=49isotope 79 Zn

Single-neutron states in the Z=30, N=49isotope 79Zn have been populated using the 78Zn(d,p)79Zn transfer reaction at REX-ISOLDE, CERN. The experimental setup allowed the combined detection of protons ejected in the reaction, and of γrays emitted by 79Zn. The analysis reveals that the lowest excited states populated in the reaction lie at approximately 1MeV of excitation, and involve neutron orbits above the N=50shell gap. From the analysis of γ-ray data and of proton angular distributions, characteristic of the amount of angular momentum transferred, a5/2+configuration was assigned to a state at 983keV. Comparison with large-scale-shell-model calculations supports a robust neutron N=50shell…

Shears Mechanism in theA∼110Region

Lifetimes of states in a rotational-like $M1$ band in ${}^{110}\mathrm{Cd}$ have been determined through a Doppler-shift attenuation method measurement performed with the Gammasphere array. The deduced $B(M1)$ values, which agree well with the predictions of the tilted axis cranking model, clearly confirm that it has the character of a shears band. Using a semiclassical scheme of the coupling of two long $j$ vectors we deduce information on the strength and form of the effective interaction between the constituent nucleons. These results are the first definitive evidence of the shears mechanism and ``magnetic rotation'' in this mass region.

Identification of excited states in 107,52Te55

Excited states in the extremely neutron-deficient nucleus 107Te have been identified from two separate experiments using the recoil-decay tagging technique. Two connected structures were observed on the basis of γγ-coincidence relations and tentatively assigned as built on the mixed-parentage νg7/2d5/2 and νh11/2 intruder configurations. The observed structures were compared with large-scale shell-model calculations and total Routhian surface calculations. Collective behavior was discovered to persist in the νh11/2 band of 107Te which highlights the shape-polarizing effect of a single valence neutron occupying the h11/2 intruder orbit as the N=50 shell closure is approached. peerReviewed

Low-spin structure of85Se and theβnbranching of85As

Fission fragments from neutron-induced fission of ${}^{235}$U produced at the high-flux reactor of the Institut Laue-Langevin, Grenoble, were separated with the Lohengrin separator to provide a beam of neutron-rich ${}^{85}\phantom{\rule{-0.16em}{0ex}}$As nuclei. The ${\ensuremath{\beta}}^{\ensuremath{-}}$ decay of ${}^{85}\phantom{\rule{-0.16em}{0ex}}$As to ${}^{85}$Se was studied using $\ensuremath{\gamma}$-$\ensuremath{\gamma}$ and $\ensuremath{\beta}$-$\ensuremath{\gamma}$ coincidence techniques. ${}^{85}$Se was also studied using the prompt-$\ensuremath{\gamma}$ coincidence data from spontaneous fission of ${}^{248}$Cm and ${}^{252}$Cf measured with the Eurogam2 and Gammasphere Ge arra…

Conversion electron spectroscopy of magnetic-rotational bands in 197Pb and 199Pb

Magnetic–rotational bands in the nearly spherical nuclei 197Pb and 199Pb and their decay to the normal states have been investigated by in–beam conversion electron spectroscopy following (heavy ion,xn) reactions. The expected M1 multipolarity of the in–band transitions has been confirmed for the strongest bands and the multipolarity of several transitions in the decay of the bands has been determined.

Electromagnetic transition rates in theN=80nucleus58138Ce

The half-life of the Iπ=6+ yrast state at Ex=2294 keV in 138Ce has been measured as T1/2=880(19) ps using the fast-timing γ-ray coincidence method with a mixed LaBr3(Ce)-HPGe array. The excited states in 138Ce have been populated by the 130Te(12C,4n) fusion-evaporation reaction at an incident beam energy of 56 MeV. The extracted B(E2;61+→41+)=0.101(24) W.u. value is compared with the predictions of truncated basis shell model calculations and with the systematics of the region. This shows an anomalous behavior compared to the neighboring isotonic and isotopic chains. Half-lives for the yrast 5-, 11+ and 14+ states in 138Ce have also been determined in this work.

Fine structure in the α decay of high-spin isomers in Lu155 and Hf156

Fine structure in the a decay of high-spin isomers in Lu-155( 25/2(-)) and Hf-156(8(+))has been studied for the first time using alpha gamma- coincidence analysis. Three new a decays from Lu-155(25 ...

Decays of theY97isomers to the single neutron nucleusZr97

The decays of the 9/2(+) and of the three-quasiparticle high spin isomer in Y-97 have been investigated following on-line mass separation with the ion-guide technique. Spins and parities for several of the lowest-lying levels in the daughter nucleus Zr-97 are revised and configurations are proposed. In particular, the 2264 keV level is identified as the h(11/2) single-neutron level. The population of a cascade on top of the h(11/2) level provides evidence for Gamow-Teller beta decay of the high-spin Y-97 isomer. Levels and transition rates are qualitatively well reproduced by regarding Zr-97 as a single-neutron nucleus with respect to the doubly closed Zr-96 core.

High-spin states beyond the proton drip-line: Quasiparticle alignments in 113 Cs

Abstract Excited states have been studied in the deformed proton emitter 113Cs. Gamma-ray transitions have been unambiguously assigned to 113Cs by correlation with its characteristic proton decay, using the method of recoil-decay tagging. Two previously identified rotational bands have been observed and extended to tentative spins of 45/2 and 51 / 2 ħ , with excitation energies over 8 MeV above the lowest state. These are the highest angular momenta and excitation energies observed to date in any nucleus beyond the proton drip-line. Transitions in the bands have been rearranged compared to previous work. A study of aligned angular momenta, in comparison to the predictions of Woods–Saxon cra…

Neutron configurations inPd113

Excited states in $^{113}\mathrm{Pd}$, populated in ${\ensuremath{\beta}}^{\ensuremath{-}}$ decay of $^{113}\mathrm{Rh}$ and in spontaneous fission of $^{248}\mathrm{Cm}$ and $^{252}\mathrm{Cf}$, have been studied by means of $\ensuremath{\gamma}$ spectroscopy at the IGISOL facility of Jyv\"askyl\"a University and using large arrays of Ge detectors (Eurogam2 and Gammasphere, respectively). The position of the ${11/2}^{\ensuremath{-}}$ yrast excitation in $^{113}\mathrm{Pd}$, proposed recently at 166.1 keV by other authors, has been corrected to 98.9 keV. The decay of this level has been discussed to explain the observed transition intensities. The ${7/2}^{\ensuremath{-}}$ member of the yras…

Precision Lifetime Measurements Using LaBr3 Detectors With Stable and Radioactive Beams

A range of high resolution gamma-ray spectroscopy measurements have been carried out using arrays which include a number of Cerium-doped Lanthanum-Tribromide (LrBr3 (Ce)) scintillation detectors used in conjunction with high-resolution hyper-pure germanium detectors. Examples of the spectral and temporal responses of such set-ups, using both standard point radioactive sources 152 Eu and 56 Co, and in-beam fusionevaporation reaction experiments for precision measurements of nuclear excited states in 34 P and 138 Ce are presented. The current and future use of such arrays at existing (EURICA at RIKEN) and future (NUSTAR at FAIR) secondary radioactive beam facilities for precision measurements…

Electromagnetic Transition Rate Measurements in theN=80 Isotone,138Ce

A study of intrinsic state halflife measurements in the N=80 nucleus 138Ce has been made using the 130Te(12C,4n)138Ce fusion evaporation reaction at beam energy of 56 MeV. The fast-timing gamma-ray coincidence method was used with a mixed LaBr3(Ce)-HPGe array to establish the lifetimes of the yrast 6+ state at 2294 keV, the Iπ=5− state at 2218 keV, the Iπ=11+ state at 3943 keV and the 14+ state at that at 5312 keV, all of which are in the sub nanosecond regime. Reduced transition probabilities have been calculated for the electromagnetic decays from these states.

Spectroscopy of Rn, Ra and Th isotopes using multi-nucleon transfer reactions

Abstract High-spin spectroscopy of Rn, Ra and Th isotopes has been performed. The nuclei have been populated using multi-nucleon transfer reactions involving a 232 Th target and a 136 Xe projectile. This type of reaction offers the only mechanism for populating high-spin states in many of these nuclei. Interleaving bands with opposite parities have been observed to high spin ( ∼28 h ) in 218,220,222 Rn, 222,224,226,228 Ra and 228,230,234 Th. A systematic study of the rotational alignment properties of octupole bands in radon, radium and thorium isotopes reveals information concerning the role of the octupole phonon and the onset of stable octupole deformation with increasing rotational freq…

Electromagnetic properties of low-lying states in neutron-deficient Hg isotopes: Coulomb excitation of Hg-182, Hg-184, Hg-186 and Hg-188

The neutron-deficient mercury isotopes serve as a classical example of shape coexistence, whereby at low energy near-degenerate nuclear states characterized by different shapes appear. The electromagnetic structure of even-mass 182-188 Hg isotopes was studied using safe-energy Coulomb excitation of neutron-deficient mercury beams delivered by the REX-ISOLDE facility at CERN. The population of $ 0^{+}_{1,2}$01,2+, $ 2^{+}_{1,2}$21,2+and $ 4^{+}_{1}$41+states was observed in all nuclei under study. Reduced E2 matrix elements coupling populated yrast and non-yrast states were extracted, including their relative signs. These are a sensitive probe of shape coexistence and may be used to validate…

Magnetic properties of smooth terminating dipole bands in 110,112Te

Three strongly coupled sequences have been established in Te-110,Te-112 up to high spins. They are interpreted in terms of deformed structures built on proton 1-particle-1-hole excitations that reach termination at I similar to 40h. This is the first observation of smooth terminating dipole structures in this mass region. Lifetime measurements have allowed the extraction of experimental B(M 1; 1 -> I - 1) and B(E2; I -> I - 2) reduced transition rates for one of the dipole bands in Te-110. The results support the deformed interpretation. (c) 2006 Elsevier B.V. All rights reserved.

Lifetime Measurements of the Neutron-RichN=30IsotonesCa50andSc51: Orbital Dependence of Effective Charges in thefpShell

The lifetimes of the first excited states of the N=30 isotones Ca-50 and Sc-51 have been determined using the Recoil Distance Doppler Shift method in combination with the CLARA-PRISMA spectrometers. This is the first time such a method is applied to measure lifetimes of neutron-rich nuclei populated via a multinucleon transfer reaction. This extends the lifetime knowledge beyond the f(7/2) shell closure and allows us to derive the effective proton and neutron charges in the fp shell near the doubly magic nucleus Ca-48, using large-scale, shell-model calculations. These results indicate an orbital dependence of the core polarization along the fp shell.

Observation of octupole structures in radon and radium isotopes and their contrasting behavior at high spin

Multinucleon transfer reactions have been used, for the first time, to populate high-spin bands of alternating parity states in {sup 218,220,222}Rn and {sup 222,224,226}Ra. The behavior of the angular momentum alignment with rotational frequency for the Rn isotopes is very different when compared with Ra and Th isotopes with N{approx}134, indicating a transition from octupole vibrational to stable octupole deformation. Throughout the measured spin range the values of {vert_bar}D{sub 0}/Q{sub 0}{vert_bar} remain constant for {sup 222}Ra and {sup 226}Ra and have a very small value for {sup 224}Ra, suggesting that the charge and mass distributions are not affected appreciably by rotations. {co…

High-spin structure of Xe134

A. Vogt et al. ; 12 págs.; 9 figs.; 1 tab.

Evolution of Octupole Deformation in Radium Nuclei from Coulomb Excitation of Radioactive Ra222 and Ra228 Beams

There is sparse direct experimental evidence that atomic nuclei can exhibit stable "pear" shapes arising from strong octupole correlations. In order to investigate the nature of octupole collectivity in radium isotopes, electric octupole (E3) matrix elements have been determined for transitions in ^{222,228}Ra nuclei using the method of sub-barrier, multistep Coulomb excitation. Beams of the radioactive radium isotopes were provided by the HIE-ISOLDE facility at CERN. The observed pattern of E3 matrix elements for different nuclear transitions is explained by describing ^{222}Ra as pear shaped with stable octupole deformation, while ^{228}Ra behaves like an octupole vibrator.

Fine structure in the α decay of Lu156 and Ta158

Smooth terminating bands inTe112: Particle-hole induced collectivity

The Gammasphere spectrometer, in conjunction with the Microball charged-particle array, was used to investigate high-spin states in Te-112 via Ni-58(Ni-58, 4p gamma) reactions at 240 and 250 MeV. Several smooth terminating bands were established, and lifetime measurements were performed for the strongest one using the Doppler-shift attenuation method. Results obtained in the spin range 18-32h yield a transition quadrupole moment of 4.0 +/- 0.5eb, which corresponds to a quadrupole deformation epsilon(2)=0.26 +/- 0.03; this value is significantly larger than the ground-state deformation of tellurium isotopes. It was also possible to extract a transition quadrupole moment for the yrast band in…

Delayed or absent π(h11/2)2 alignment in Xe111

First Exploration of Neutron Shell Structure below Lead and beyond N=126

The nuclei below lead but with more than 126 neutrons are crucial to an understanding of the astrophysical r process in producing nuclei heavier than A∼190. Despite their importance, the structure and properties of these nuclei remain experimentally untested as they are difficult to produce in nuclear reactions with stable beams. In a first exploration of the shell structure of this region, neutron excitations in ^{207}Hg have been probed using the neutron-adding (d,p) reaction in inverse kinematics. The radioactive beam of ^{206}Hg was delivered to the new ISOLDE Solenoidal Spectrometer at an energy above the Coulomb barrier. The spectroscopy of ^{207}Hg marks a first step in improving our…

Shears mechanism in109Cd

Lifetimes of high-spin states in two $\ensuremath{\Delta}I=1$ bands and one $\ensuremath{\Delta}I=2$ band in ${}^{109}\mathrm{Cd}$ have been measured using the Doppler shift attenuation method in an experiment performed using the ${}^{96}\mathrm{Zr}{(}^{18}\mathrm{O},5n)$ reaction with the GAMMASPHERE array. Experimental total angular momenta and reduced transition strengths for both $\ensuremath{\Delta}I=1$ bands were compared with tilted axis cranking (shears mechanism) predictions and the $\ensuremath{\Delta}I=2$ band with principal axis cranking predictions, based on configurations involving two proton ${g}_{9/2}$ holes and one or three valence quasineutrons from the ${h}_{11/2}$ and mi…

High-spin states of $^{218}$Th

Abstract High-spin states in the N = 128 nucleus 218Th have been investigated following fusion–evaporation reactions, using the recoil-decay tagging technique. Due to the short-lived nature of the ground state of 218Th prompt γ rays have been correlated with the α decay of the daughter nucleus 214Ra. The level scheme representing the decay of excited states has been extended to (16+) with the observation of six previously unreported transitions. The observations are compared with the results of shell model calculations and within the context of the systematics of neighbouring nuclei.

Interaction position resolution simulations and in-beam measurements of the AGATA HPGe detectors

WOS: 000290082600015

High-spin states in the neutron-rich A∼100 region

Two experimental setups have been used to study excited states of neutron‐rich nuclei in the A∼100 region. Extended level schemes and lifetime measurements were obtained using deep‐inelastic and fusion‐fission reactions with the CLARA‐PRISMA spectrometer and the Ge‐array GASP respectively. Experimental information from GASP has been used to complement the CLARA‐PRISMA experiment. Time spectra have been used to measure the lifetimes of isomeric states. Preliminary results are presented for 89Rb.

The observation of vibrating pear-shapes in radon nuclei

6 pags., 4 fig.s, 1 tab. -- Open Access funded by Creative Commons Atribution Licence 4.0

Excited states in 217Ra populated in the α decay of 221Th

Fine structure in the α decay of 22190Th, populating excited states in 21788Ra, was studied using αγ-coincidence spectroscopy. Two α-decay branches from 221Th have been newly observed, with Eα(keV)[bα(%)]=7951(8)[0.14(3)] and 8247(3)[1.51(12)], together with three previously known branches. Also, two new states in 217Ra were identified at E = 177 and 227 keV. The ground-state configurations of the odd-A, N = 131 transitional isotones above 208Pb are interpreted from their α-decay fine structure systematics and considered in terms of predictions using spherical shell and reflection-asymmetric models. peerReviewed

α-decay spectroscopy of the N = 130 isotones 218Ra and 220Th: Mitigation of α-particle energy summing with implanted nuclei

An analysis technique has been developed in order to mitigate energy summing due to sequential short-lived α decays from nuclei implanted into a silicon detector. Using this technique, α-decay spectroscopy of the N=130 isotones 218Ra (Z=88) and 220Th (Z=90) has been performed. The energies of the α particles emitted in the 218Ra→214Rn and 220Th→216Ra ground-state-to-ground-state decays have been measured to be 8381(4) keV and 8818(13) keV, respectively. The half-lives of the ground states of 218Ra and 220Th have been measured to be 25.99(10) μs and 10.4(4) μs, respectively. The half-lives of the ground states of the α-decay daughters, 214Rn and 216Ra, have been measured to be 259(3) ns and …

Delayed or absent π(h11/2)2 alignment in 111Xe

Excited states have been identified in the very neutron-deficient N = Z + 3 nucleus 111Xe for the first time, using the 58Ni(58Ni, αn) heavy-ion fusion-evaporation reaction. γ -ray transitions have been unambiguously assigned to 111Xe by correlation with the characteristic 111Xe → 107Te → 103Sn α-decay chain using the method of recoil-decay tagging. Inspection of γ γ -coincidence data has shown that five of the transitions form a rotational-like sequence. Excitation-energy systematics suggest that the sequence could be the favored signature partner of a band built on an h11/2 neutron. Aligned angular momenta of states in the band have been compared to analogous bands in neighboring xenon is…

Deformation of the proton emitterCs113from electromagnetic transition and proton-emission rates

The lifetime of the $(11/{2}^{+})$ state in the band above the proton-emitting $(3/{2}^{+})$ state in $^{113}\mathrm{Cs}$ has been measured to be $\ensuremath{\tau}=24(6)$ ps from a recoil-decay-tagged differential-plunger experiment. The measured lifetime was used to deduce the deformation of the states using wave functions from a nonadiabatic quasiparticle model to independently calculate both proton-emission and electromagnetic $\ensuremath{\gamma}$-ray transition rates as a function of deformation. The only quadrupole deformation, which was able to reproduce the experimental excitation energies of the states, the electromagnetic decay rate of the $(11/{2}^{+})$ state and the proton-emis…

Single-particle states and parity doublets in odd-Z 221Ac and 225Pa from α-decay spectroscopy

Low-lying states in the odd-Z isotopes 22189Ac132 and 22591Pa134 have been studied using α-particle and αγ-coincidence spectroscopy in the 225Pa→221Ac→217Fr decay chain. Ground-state spin and parity assignments of Iπ = 5/2− are proposed for both 221Ac and 225Pa, with the odd proton occupying the Ω = 5/2 orbital of the quadrupole-octupole deformed shell model in both nuclei. In 221Ac, excited states in the bands based on the Ω = 5/2 and Ω = 3/2 orbitals have been identified, including proposed parity-doublet states. The results suggest that reflection-asymmetric deformation of the ground state persists in the odd-A members of the isotope chains down to N = 132 for Ac and N = 134 for Pa, befo…

High-spin structure in the transitional nucleus Xe131 : Competitive neutron and proton alignment in the vicinity of the N=82 shell closure

The transitional nucleus 131Xe is investigated after multinucleon transfer (MNT) in the 136Xe+208Pb and 136Xe+238U reactions employing the high-resolution Advanced GAmma Tracking Array (AGATA) coupled to the magnetic spectrometer PRISMA at the Laboratori Nazionali di Legnaro, Italy and as an elusive reaction product in the fusion-evaporation reaction 124Sn(11B,p3n) 131Xe employing the HORUS γ-ray array coupled to a double-sided silicon strip detector (DSSSD) at the University of Cologne, Germany. The level scheme of 131Xe is extended to 5 MeV. A pronounced backbending is observed at ~ω ≈ 0.4 MeV along the negative-parity one-quasiparticle νh11/2(α = −1/2) band. The results are compared to t…

AGATA-Advanced GAmma Tracking Array

WOS: 000300864200005

Coulomb excitation of pear-shaped nuclei

There is a large body of evidence that atomic nuclei can undergo octupole distortion and assume the shape of a pear. This phenomenon is important for measurements of electric-dipole moments of atoms, which would indicate CP violation and hence probe physics beyond the Standard Model of particle physics. Isotopes of both radon and radium have been identified as candidates for such measurements. Here, we have observed the low-lying quantum states in 224Rn and 226Rn by accelerating beams of these radioactive nuclei. We show that radon isotopes undergo octupole vibrations but do not possess static pear-shapes in their ground states. We conclude that radon atoms provide less favourable condition…