0000000000919823
AUTHOR
G. Münzenberg
From nuclear halos to superheavy nuclei—Perspectives for nuclear structure research at GSI
Of fundamental interest is the investigation of nuclear matter at the limits of its existence in the vicinity of the driplines and in the region of the superheavy elements. The availability of unstable nuclei over large energy ranges and new experimental developments gave new impulse to nuclear structure research. Examples are the investigations of halo nuclei by nuclear decay studies combined with reactions at low and high energies, the mapping of the mass surface in large-scale direct mass measurements, and the production of heavy and superheavy nuclei. New developments such as high-current accelerators or the next generation of radioactive beam facilities will lead to further progress in…
Low-energy fission investigated in reactions of 750 AMeV 238U-ions with Pb and Be targets
Charge distributions of fragments from low energy nuclear fission are investigated in reactions of highly fissile238U projectiles at relativistic energies (750 A·MeV) with a heavy (Pb) and a light (Be) target. The fully stripped fission fragments are separated by the Fragment Separator (FRS). Their high kinetic energies in the laboratory system allow the identification of all atomic numbers by using Multiple-Sampling Ionization Chambers (MUSIC). The elemental distributions of fragments observed at larger magnetic rigidities than the238U projectiles show asymmetric break-up and odd-even effects. They indicate a low energy fission process, induced mainly by dissociation in the electro-magneti…
Three-body correlations in electromagnetic dissociation of Borromean nuclei: The 6He case
20 pages, 2 tables, 9 figures, 1 appendix.-- PACS nrs.: 25.60.-t; 27.20.+n; 25.70.De; 25.75.Gz.-- Printed version published Sep 5, 2005.
The new nuclide225U
In the bombardment of a 270μg/cm 2 180Hf target with48 Ca projectiles at a primary beam energy of E/A=4.24 MeV/u the new nuclide225U was produced. The experiment was performed at the velocity filter SHIP. 225U was found to decay by α emission with Eα=(7880 ±20) keV (≈90%), (7830±20) keV (≈10%) and has a half-life ofT 1/2=(80 −20 +40 ms).
Invariant mass spectrum and α-n correlation function studied in the fragmentation of 6He on a carbon target
13 pags, 5 figures.-- PACS nrs.: 24.60.−t; 25.70.Ef; 27.20.+n.
Measurements of the dipole response with radioactive beams
Super Heavy Elements - experimental developments
With his theoretical work Walter Greiner, our mentor, pioneered super heavy element research and motivated us young scientists. He actively shaped the profile of GSI. We are happy that still during his lifetime we could prove some of his predictions: Fusion with magic nuclei paving the way to super heavy elements and the proof of the prediction of the nuclear species existing only by shell stabilization, super heavy elements. With the discovery of oganesson, Z=118, the heaviest element known today, we have come to the end of this era. New experimental developments will be discussed.
Systematic investigation of the drip-line nuclei 11Li and 14Be and their unbound subsystems 10Li and 13Be
Fragmentation reactions in a carbon target with beams of 11Li and 14Be at relativistic energies have been studied in a kinematically complete experiment at the ALADIN-LAND setup at GSI. Excited states in 11Li and 14Be were obtained from the data in the inelastic channel. The measured cross sections with the core nucleus in the final state show that in the 14Be case core polarization plays an important role. In the one-neutron knockout channels the measured angular correlations between fragment and neutron are asymmetric, which demonstrates the presence of states with different parities in the 11Li and 14Be ground states. For 10Li a low-lying virtual s-state, a p-state and evidence for a d-s…
Multi-nucleon transfer reactions at ion catcher facilities : a new way to produce and study heavy neutron-rich nuclei
Abstract The production of very neutron-rich nuclides heavier than fission fragments is an ongoing experimental challenge. Multi-nucleon transfer reactions (MNT) have been suggested as a method to produce these nuclides. By thermalizing the reaction products in gas-filled stopping cells, we can deliver them as cooled high-quality beams to decay, laser and mass spectrometry experiments. High precision mass spectrometry will allow for the first time to universally and unambiguously identify the atomic and proton numbers of the ions produced in MNT reactions. In this way their ground and isomeric state properties can be studied in high-precision measurements. In experiments at IGISOL, Finland …
Walter Greiner, a Pioneer in Super Heavy Element Research Historical Remarks and New Experimental Developments
With his theoretical work Walter Greiner pioneered super-heavy element research. He motivated the young scientists and actively shaped the profile of the Gesellschaft fur SchwerIonenforschung, GSI, Darmstadt. We are happy that still during his lifetime we at GSI could prove some of his predictions: Fusion with magic nuclei and super heavy elements, the nuclear species existing only by shell stabilization. With the discovery of oganesson, Z = 118, the heaviest element known today, we have come to the end of super heavy-element production by the fusion of magic nuclei. In-flight separation and new experimental developments including Walter Greiner’s new ideas for SHE synthesis will be discuss…
Few-neutron removal from238U at relativistic energies
As part of a comprehensive study of uranium fragmentation at relativistic energies at the GSI projectile fragment separator, FRS, inclusive neutron-removal cross sections have been measured for severalxn channels at projectile energies of 600 and 950A MeV using targets of Al, Cu and Pb. The variation of the experimental cross sections with target nuclear charge is used to disentangle nuclear and electromagnetic contributions. The electromagnetic cross sections agree surprisingly well with a simple harmonic oscillator calculation of giant dipole resonances based on measured photonuclear cross sections and do not require an extra enhancement of the two-phonon giant dipole excitation as conclu…
Mass measurement of cooled neutron-deficient bismuth projectile fragments with time-resolved Schottky mass spectrometry at the FRS-ESR facility
Masses of 582 neutron-deficient nuclides ($30\leq{Z}\leq{85}$) were measured with time-resolved Schottky mass spectrometry at the FRS-ESR facility at GSI, 117 were used for calibration. The masses of 71 nuclides were obtained for the first time. A typical mass accuracy of 30 $\mu$u was achieved. These data have entered the latest atomic mass evaluation. The mass determination of about 140 additional nuclides was possible via known energies ($Q$-values) of $\alpha-$, $\beta-$, or proton decays. The obtained results are compared with the results of other measurements.
Exclusive measurement of breakup reactions with the one-neutron halo nucleus11Be
Electromagnetic and nuclear inelastic scattering of the halo nucleus ${}^{11}\mathrm{Be}$ have been investigated by a measurement of the one-neutron removal channel, utilizing a secondary ${}^{11}\mathrm{Be}$ beam with an energy of 520 MeV/nucleon impinging on lead and carbon targets. All decay products, i.e., ${}^{10}\mathrm{Be}$ fragments, neutrons, and $\ensuremath{\gamma}$ rays have been detected in coincidence. Partial cross sections for the population of ground and excited states in ${}^{10}\mathrm{Be}$ were determined for nuclear diffractive breakup as well as for electromagnetically induced breakup. The partial cross sections for ground-state transitions have been differentiated fur…
Fine structure in a alpha decay of 188, 192Po
The α decay of 188,192Po has been reexamined in order to probe the 0+ states in the daughter nuclei 184,188Pb that can be associated with coexisting spherical, oblate, and∕or prolate configurations. Improved values were measured for the excitation energy and the feeding α-decay intensity of the 0+2state in 184,188Pb and conflicting results on the 0+3 state in 188Pb were clarified. All known cases of fine structure in the α decay of the even-even Po nuclei are reviewed. The reduced α-decay width systematics combined with potential-energy-surface calculations confirm the onset of deformation in the ground state of the polonium nuclei around the neutron midshell. An isomeric state with a half-…
STUDIES OF SUPERHEAVY ELEMENTS AT SHIP
An overview of present experimental investigation of superheavy elements is given. The data are compared with theoretical descriptions. Results are reported from an experiment to confirm production of element 112 isotopes in irradiation of 238 UF 4 with 48 Ca . One spontaneous fission event was measured, which agrees with three events of previously measured data which had been assigned to the decay of 283112. However, more experimental work is needed in order to obtain an independent and unambiguous confirmation of previous results.
Development of quadrupole collectivity in the neutron-rich Ni, Zn, Ge, and Se isotopes
An experiment was performed to study the collective properties of neutron-rich Ni, Zn, Ge, and Se isotopes. Of particular interest is the vicinity of the N = 50 and Z = 28 shell closures. For most neutron-rich nuclei in this region of the chart of nuclei the B(E2) values of the transitions from the ground to the first excited 2+ states are unknown. This information would give valuable insight into the changes in nuclear structure when going to more neutron-rich nuclei.
Two- and three-body correlations: breakup of halo nuclei
4 pages, 2 figures.
Determination of the partial electron capture- and spontaneous-fission half-lives of254No
The isotope254No was produced in the fusion reaction48Ca +208Pb. Using the velocity filter SHIP and radiochemical techniques it was found that the nuclide254No with a half-life of 55 s decays byα, EC, and spontaneous-fission. Deduced partial half-lives are (61±2) s forα-decay, (550−160+370) s for EC and [2.2−1.0+2.0]×104 s for spontaneous fission.
Alpha decay of the new isotopes 188,189Po
New neutron-deficient isotopes 188,189Po have been produced in the complete fusion reaction of 52Cr ions with a 142Nd target at the velocity filter SHIP. The evaporation residues were separated in-flight and subsequently identified on the basis of α-γ and α-conversion electron coincidence measurements and of α-α position and time correlations. In 189Po a ground state to ground state α decay with Eα1= 7540(20) keV, T1/2= 5(1) ms and two fine structure α-decays at Eα2= 7264(15) keV and Eα3= 7316(15) keV have been observed. In 188Po (T1/2= 400+200 −150μs) a ground state to ground state α decay at Eα= 7915(25) keV and a fine structure α decay at Eα= 7350(40) keV have been found. Improved data o…
Lithium isotopes beyond the drip line
The unbound isotopes 10Li, 12Li and 13Li have been observed after nucleon-knockout reactions at relativistic energies with 11Li and 14Be beams impinging on a liquid hydrogen target. The channels , and were analysed in the ALADIN-LAND setup at GSI. The 10Li data confirm earlier findings, while the 12Li and 13Li nuclei were observed for the first time. The relative-energy spectrum shows that the ground state of 12Li can be described as a virtual s-state with a scattering length of -13.7(1.6) fm. A broad energy spectrum was found for the channel. Based on the assumption that the relative-energy spectrum is dominated by a correlated background presumably stemming from initial correlations in th…
Observation of a dramatic hindrance of the nuclear decay of isomeric states for fully ionized atoms
Abstract The half-lives of isomeric states of fully ionized 144Tb, 149Dy and 151Er have been measured. These nuclides were produced via fragmentation of about 900 MeV/u 209Bi projectiles, separated in flight with the fragment separator (FRS) and stored in the cooler ring (ESR). The decay times of the cooled fragments have been measured with time-resolved Schottky spectrometry. We observed for the first time drastic increases of the half-lives of bare isomers by factors of up to 30 compared to their neutral counterparts. This is due to the exclusion of the strong internal conversion and electron-capture channels in the radioactive decay of these bare nuclei. The experimental results are in g…
Energy and range focusing of in-flight separated exotic nuclei – A study for the energy-buncher stage of the low-energy branch of the Super-FRS
Abstract The relative momentum spread of in-flight separated exotic nuclear beams produced in fragmentation and/or fission reactions is of the order of a few percent. A new technique is presented, which reduces the momentum spread significantly, and first experimental results obtained with relativistic projectile fragments are shown. This technique is the key to experiments with slowed-down and stopped beams, in particular for the efficient stopping of relativistic exotic nuclei in gas-filled stopping cells. It will be employed at the energy-buncher stage of the low-energy branch of the Super-FRS facility. The ion-optical design of the energy buncher is presented and a brief outlook to the …
The new element 112
The new element 112 was produced and identified unambiguously in an experiment at SHIP, GSI Darmstadt. Two decay chains of the isotope277112 were observed in irradiations of208Pb targets with70Zn projectiles of 344 MeV kinetic energy. The isotope decays by emission of α particles with a half-life of (240 −90 +430 )µs. Two different α energies of (11,649±20) keV and (11,454±20) keV were measured for the two observed decays. The cross-section measured in three weeks of irradiations is (1.0 −0.4 +1.8 ) pb.
Coulomb breakup of psd-shell neutron-rich nuclei
Inelastic scattering of loosely bound nuclei by Coulomb interaction at intermediate energies (400?600 MeV/nucleon) has been utilized as a spectroscopic tool for exotic nuclei. The observed electromagnetic dipole (E1) strength above the one neutron threshold of neutron-rich C, Be, B and O isotopes can be explained by a non-resonant transition of a neutron into the continuum. The shape of these strength distributions reflects properties of the wavefunction of the released neutron in the nucleus and hence ground-state properties of these isotopes. Neutron capture cross-sections such as for the 14C(n,?) 15C reaction which are of astrophysical relevance can be deduced indirectly.
Continuum excitations in6He
T. Aumann et al. ; 11 pags.; 6 figs.; 2 tabs. ; PACS number(s): 27.20.1n, 25.60.Gc, 25.70.De, 29.30.Hs
First spatial isotopic separation of relativistic uranium projectile fragments
Abstract Spatial isotopic separation of relativistic uranium projectile fragments has been achieved for the first time. The fragments were produced in peripheral nuclear collisions and spatially separated in-flight with the fragment separator FRS at GSI. A two-fold magnetic-rigidity analysis was applied exploiting the atomic energy loss in specially shaped matter placed in the dispersive central focal plane. Systematic investigations with relativistic projectiles ranging from oxygen up to uranium demonstrate that the FRS is a universal and powerful facility for the production and in-flight separation of monoisotopic, exotic secondary beams of all elements up to Z = 92. This achievement has …
The new element 111
The new element 111 was produced and unambiguously identified in an experiment at SHIP, GSI Darmstadt. Three nuclei of the isotope272111 were observed in irradiations of209Bi targets with64Ni projectiles of 318 MeV and 320 MeV energy. The cross-sections are (1.7 −1.4 +3.3 ) pb and (3.5 −2.3 +4.6 ) pb, respectively. The nuclei decay by a emission into the new and so far the heaviest isotopes of the elements 109 and 107 with mass numbers A=268 and A=264. Theα-decay chains were followed down to the known nuclei260105 and256Lr.
Coulomb breakup of 23O
Abstract The ground-state structure of the near-drip-line nucleus 23O has been investigated in a one-neutron Coulomb breakup reaction. Differential cross sections d σ / d E * for electromagnetic excitation of 23O projectiles (422 MeV/nucleon) incident on a lead target have been obtained from the measurement of the momenta of all breakup products including γ rays. The analysis of the deduced dipole-transition probability into the continuum infers a 2 s 1 / 2 ⊗ O 22 ( 0 + ) ground state configuration with a spectroscopic factor of 0.77(10) and thus a ground-state spin I π ( O 23 ) = 1 / 2 + , resolving earlier conflicting experimental findings. Final-state interaction is of significant influe…
New results on elements 111 and 112
Experiments on the synthesis and identification of the nuclei 272111 and 277112 were performed in order to confirm previous results. Three additional decay chains were measured in the reaction 64Ni + 209Bi →273111*. The study revealed considerably improved data on the decay chain originating from 272111. One additional chain was measured in the reaction 70Zn + 208Pb →278112*. The decay properties of the chain starting at 277112 are in excellent agreement with the second chain of the first experiment down to 265Sg, where the new chain ends by a previously unknown spontaneous-fission branch. A re-analysis of all the data on elements 110, 111, and 112 measured at GSI since 1994 (a total of 34 …
β-delayed fission of186,188Bi isotopes
By using the technique of correlating implanted evaporation residues and their subsequent fission decay, $\ensuremath{\beta}$-delayed fission ($\ensuremath{\beta}$DF) of ${}^{186}$Bi has been identified for the first time and $\ensuremath{\beta}$DF of ${}^{188}$Bi has been unambiguously confirmed. The experiments were performed at the velocity filter SHIP (GSI, Darmstadt). The $\ensuremath{\beta}$DF probabilities for both nuclides were qualitatively estimated, and, in particular indications for a large value in the case of ${}^{186}$Bi are regarded.
α-decay spectroscopy of the new isotopeAt192
Decay properties of the new neutron-deficient nuclide $^{192}\mathrm{At}$ have been studied in the complete fusion reaction $^{144}\mathrm{Sm}$($^{51}\mathrm{V}$,3n)$^{192}\mathrm{At}$ at the velocity filter SHIP. Two isomeric states with half-lives of 88(6) ms and 11.5(6) ms, respectively, and with complex $\ensuremath{\alpha}$-decay schemes were identified in $^{192}\mathrm{At}$. The decay pattern of one of the isomers suggests that it is based on the oblate-deformed $\ensuremath{\pi}2{f}_{7/2}\ensuremath{\bigotimes}\ensuremath{\nu}1{i}_{13/2}$ configuration, which confirms the expected onset of deformation in the At isotopes by approaching the neutron midshell at $N=104$.
Giant resonances in unstable oxygen isotopes
Abstract Electromagnetic and nuclear breakup of the neutron-rich Oxygen isotopes ranging from A = 17 to A = 22 is studied experimentally in reactions at energies around 600 MeV/u. The beams were produced in fragmentation reactions and separated by the GSI Fragment Separator FRS. By measuring the four-momenta of all decay products after inelastic scattering and neutron decay of the projectile, the excitation energy is determined. From the differential cross sections dσ dE ∗ for electromagnetic excitation, the E1-strength distributions can be deduced. For 18,20,22O, low-lying dipole strength is observed, exhausting about 5% of the Thomas Reiche Kuhn sumrule for energies up to 5 MeV above the …
Production and decay of269110
In an experiment carried out to identify element 110, we have observed anα-decay chain, that can be unambiguously assigned to269110. In a scries of preexperiments the excitation functions of the fusion reactions50Ti +208Pb→258104* and58Fe +208Pb→266108* were measured with high precision in order to get the optimum projectile energies for the production of these heavy elements. The cross-section maxima of the 1n evaporation channels were observed at excitation energies of 15.6 MeV and 13.4 MeV, respectively. These data result in an optimum excitation energy of 12.3 MeV of the compound nucleus for the production of269110 in the reaction62Ni +208Pb→269110 + 1n. In irradiations at the correspon…
First isochronous mass spectrometry at the experimental storage ring ESR
Short-lived exotic nuclei can be produced and separated with the high-energy secondary nuclear beam facility FRS at GSI. These nuclides can be injected and stored in the storage ring ESR. The lower lifetime limit of the presently existing methods for mass measurements on these nuclides at the ESR is about a few seconds. We have developed and investigated an isochronous operational mode of the ESR, that makes mass measurements of nuclides with lifetimes down to a few ls feasible. It has been commissioned in experiments using long-lived nuclides with known masses. A mass resolving power of about 150 000 has been achieved in a "rst pilot experiment. A suitable detector system has been implemen…
Influence of Collective Surface Motion on the Threshold Behavior of Nuclear Fusion
Fusion excitation functions for the systems $^{40}\mathrm{Ar}$+$^{112,116,122}\mathrm{Sn}$ and $^{40}\mathrm{Ar}$+$^{144,148,154}\mathrm{Sm}$ have been determined, covering cross sections ranging from several hundred millibarns down to the microbarn level. The data are interpreted with a fusion model that includes fluctuations of the barrier with an amplitude that is shown to be correlated with the collective surface properties of the nuclei. There is no need to assume an additional enhanced tunneling process.
Searching for the 5H resonance in the t+n+n system
19 pages, 7 figures, 2 tables, 2 appendices.-- PACS nrs.: 27.10.+h; 25.60.Gc.-- Printed version published Jul 28, 2003.
Cross section systematics for the lightest Bi and Po nuclei produced in complete fusion reactions with heavy ions
The production of the very neutron-deficient nuclides $^{184\ensuremath{-}192}\mathrm{Bi}$ and $^{186\ensuremath{-}192}\mathrm{Po}$ in the vicinity of the neutron midshell at N = 104 has been studied by using heavy-ion-induced complete fusion reactions in a series of experiments at the velocity filter SHIP. The cross sections for the xn and pxn evaporation channels of the $^{46}\mathrm{Ti}$+$^{144}\mathrm{Sm}$$\ensuremath{\rightarrow}^{190}\mathrm{Po}{}^{*},$$^{98}\mathrm{Mo}$+$^{92}\mathrm{Mo}$$\ensuremath{\rightarrow}^{190}\mathrm{Po}{}^{*},$$^{50,52}\mathrm{Cr}$+$^{142}\mathrm{Nd}$$\ensuremath{\rightarrow}^{192,194}\mathrm{Po}{}^{*}$, and $^{94,95}\mathrm{Mo}$+$^{93}\mathrm{Nb}$$\ensurem…
Cold fusion of heavy ions paving the way to superheavy elements
Abstract Significant progress has been made approaching superheavy elements. A shell-stabilized region near hassium has been discovered. Element 112 has been synthesized. Recently evidence for the creation of elements 114, 116, and 118 has been reported. The way to these superheavy nuclei was paved by the cold fusion of heavy ions. In this paper experimental methods for heavy-element research, which is essentially physics with single atoms, are presented together with recent experimental results. The observed nuclear properties are discussed in the framework of theoretical models. New instrumental developments including accelerators and radioactive beams are be addressed.
Probing intruder structures in lead nuclei
In-beam γ-ray spectroscopy measurements provide important information on coexisting normal and intruder configurations in lead nuclei. However, in these experiments the yrast states are preferentially populated so that in many cases nothing is known about non-yrast states that are essential for obtaining a fuller understanding. Complementary experiments designed to study fine structure in the a decays of polonium nuclei have led to the discovery of low-spin non-yrast states in the daughter lead nuclei, while higher-spin states can be identified through the γ decays of isomeric states. The α-decay studies have the additional benefit of allowing information on configuration mixing in the polo…
The electronion scattering experiment ELISe at the International Facility for Antiproton and Ion Research (FAIR) - A conceptual design study
The electronion scattering experiment ELISe is part of the installations envisaged at the new experimental storage ring at the International Facility for Antiproton and Ion Research (FAIR) in Darmstadt, Germany. It offers an unique opportunity to use electrons as probe in investigations of the structure of exotic nuclei. The conceptual design and the scientific challenges of ELISe are presented. © 2011 Elsevier B.V. All rights reserved.
Radioactive beams at GSI
Abstract After a brief introduction the production of relativistic beams of exotic nuclei will be discussed and some characteristic examples from the ongoing GSI nuclear structure research programme are presented, such as: nuclear reactions with exotic beams to explore nuclear skins, the structure of halo nuclei, and direct mass measurements in a storage ring. Heavy-element research will be addressed briefly. A possible next generation exotic beam facility at GSI will be outlined.
Photoneutron cross sections for unstable neutron-rich oxygen isotopes.
The dipole response of stable and unstable neutron-rich oxygen nuclei of masses A = 17 to A = 22 has been investigated experimentally utilizing electromagnetic excitation in heavy-ion collisions at beam energies about 600 MeV/nucleon. A kinematically complete measurement of the neutron decay channel in inelastic scattering of the secondary beam projectiles from a Pb target was performed. Differential electromagnetic excitation cross sections d sigma/dE were derived up to 30 MeV excitation energy. In contrast to stable nuclei, the deduced dipole strength distribution appears to be strongly fragmented and systematically exhibits a considerable fraction of low-lying strength.
Invariant-mass spectroscopy of $^{10}$Li and $^{11}$Li
Break-up of secondary Li-11 ion beams (280 MeV/nucleon) on C and Pb targets into Li-9 and neutrons is studied experimentally. Cross sections and neutron multiplicity distributions are obtained, characterizing different reaction mechanisms. Invariant-mass spectroscopy for Li-11 and Li-10 is performed. The E1 strength distribution, deduced from electromagnetic excitation of Li-11 up to an excitation energy of 4 MeV comprises similar to 8% of the Thomas-Reiche-Kuhn energy-weighted sumrule strength. Two low-lying resonance-like structures are observed for Li-10 at decay energies of 0.21(5) and 0.62(10) MeV, the former one carrying 26(10)% of the strength and likely to be associated with an s-wa…
Neutron momentum distributions from "core break-up" reactions of halo nuclei
Neutron angular distributions from violent break-up reactions of Li-11 and Be-11 have been measured at 28 MeV/u and 280 MeV/u and at 41 MeV/u and 460 MeV/u, respectively. The derived neutron momentum distributions show a narrow component in transverse momentum that is within uncertainties independent of beam energy and target charge. This component is suggested to be simply related to the momentum distribution of the loosely bound halo neutron(s) in the projectiles.
Simultaneous Measurement ofβ−Decay to Bound and Continuum Electron States
We report the first measurement of a ratio {lambda}{sub {beta}{sub b}}/{lambda}{sub {beta}{sub c}} of bound-state ({lambda}{sub {beta}{sub b}}) and continuum-state ({lambda}{sub {beta}{sub c}}) {beta}{sup -}-decay rates for the case of bare {sup 207}Tl{sup 81+} ions. These ions were produced at the GSI fragment separator FRS by projectile fragmentation of a {sup 208}Pb beam. After in-flight separation with the B{rho}-{delta}E-B{rho} method, they were injected into the experimental storage-ring ESR at an energy of 400.5A MeV, stored, and electron cooled. The number of both the {sup 207}Tl{sup 81+} ions and their bound-state {beta}{sup -}-decay daughters, hydrogenlike {sup 207}Pb{sup 81+} ion…
High-power production targets for the Super-FRS using a fast extraction scheme
Abstract The high-power production target of the Super-FRS [H. Geissel et al., these Proceedings] will be irradiated by very intense heavy-ion beams which will be delivered from the future SIS100/200 [An International Accelerator Facility for Beams of Ions and Antiprotons, GSI-Report, 2001] synchrotron facility at the Gesellschaft fur Schwerionenforschung (GSI) Darmstadt. This paper presents calculations of the thermodynamic and the hydrodynamic response of such a target, considering that a uranium ion beam with an energy of 1 GeV/u and an intensity of 10 12 particles will impinge within 50 ns on a solid carbon target with a thickness of 4 g/cm 2 . Due to the high beam intensity the target …
Decay properties of neutron-deficient isotopes 256, 257Db, 255Rf, 252, 253Lr
Isotopes of dubnium (element 105) with mass numbers A = 256, 257, and 258 were produced by the reaction 209Bi(50Ti,xn) 259-xDb (x = 1, 2, 3) at projectile energies of (4.59-5.08) AMeV. Excitation functions were measured for the 1n, 2n and 3n evaporation channels. The same position of the excitation function was observed for the 1n channel as for the previously measured 1n channel of the reaction 208Pb(50Ti,1n)257Rf. The measured α-decay data of 257Db and its daughter products resulted in the identification of α-decaying isomeric states in 257Db and 253Lr. Two new isotopes, 256Db and 252Lr, were produced at the highest bombarding energies of 4.97 AMeV and 5.08 AMeV. They were identified by d…
Measurement of the dipole response of neutron-rich nuclei in the A∼20 region
Abstract Coulomb break up of the neutron-rich 15,17 C and 17–22 O isotopes has been studied experimentally using secondary beams at energies of 500–600 MeV/u. A comparison between differential cross sections, d σ/ d E ∗ , with that obtained from a binary model shows that the main ground-state configuration of 15 C is 14 C(0 + )⊗ ν S 1/2 as expected. For 17 C, our preliminary data analysis reveals that the predominant (∼64%) configuration of the ground state is 16 C(2 + )⊗ ν s , d . For 17–22 O, the low-lying E1 strength amounts up to about 12% of the energy weighted sum rule strength depending on neutron number. The energy weighted E1 strength (integrated up to 15 MeV excitation energy) inc…
α-decay of the new isotopePo187: Probing prolate structures beyond the neutron mid-shell at N = 104
The new neutron-deficient isotope $^{187}\mathrm{Po}$ has been identified in the complete fusion reaction $^{46}\mathrm{Ti}$+$^{144}\mathrm{Sm}$\ensuremath{\rightarrow}$^{187}\mathrm{Po}$+$3n$ at the velocity filter SHIP. Striking features of the $^{187}\mathrm{Po}$ \ensuremath{\alpha} decay are the strongly-hindered decay to the spherical ground state and unhindered decay to a surprisingly low-lying deformed excited state at 286 keV in the daughter nucleus $^{183}\mathrm{Pb}$. Based on the potential energy surface calculations, the $^{187}\mathrm{Po}$ ground state and the 286 keV excited state in $^{183}\mathrm{Pb}$ were interpreted as being of prolate origin. The systematic deviation of t…
Dissociation of 8He into 6He + n + X at 240 MeV/u
4 pages, 3 figures, 2 tables.
Fragmentation of exotic oxygen isotopes
Abrasion-ablation models and the empirical EPAX parametrization of projectile fragmentation are described. Their cross section predictions are compared to recent data of the fragmentation of secondary beams of neutron-rich, unstable 19,20,21O isotopes at beam energies near 600 MeV/nucleon as well as data for stable 17,18O beams.
A triplet of differently shaped spin-zero states in the atomic nucleus 186Pb
Understanding the fundamental excitations of many-fermion systems is of significant current interest. In atomic nuclei with even numbers of neutrons and protons, the low-lying excitation spectrum is generally formed by nucleon pair breaking and nuclear vibrations or rotations. However, for certain numbers of protons and neutrons, a subtle rearrangement of only a few nucleons among the orbitals at the Fermi surface can result in a different elementary mode: a macroscopic shape change. The first experimental evidence for this phenomenon came from the observation of shape coexistence in 16O (ref. 4). Other unexpected examples came with the discovery of fission isomers and super-deformed nuclei…
New results with stored exotic nuclei at relativistic energies
Recently, much progress has been made with stored exotic nuclei at relativistic velocities ( v c = 0.7 ) . Fragments of 208Pb and 209Bi projectiles and fission products from 238U ions were produced, separated in flight with the fragment separator FRS, and injected into the storage-cooler ring ESR for precision measurements. 114 new masses of neutron-deficient isotopes in the lead region have been measured with time-resolved Schottky Mass Spectrometry (SMS). A new isospin dependence of the pairing energy was observed due to the improved mass accuracy of typically 1.5×10-7 (30 keV). New masses of short-lived neutron-rich fission fragments have been obtained with Isochronous Mass Spectrometry …
Study of Basic Nuclear Properties of Highly-Charged, Unstable Nuclei at the SIS-FRS-ESR Complex
Recent progress in experiments with exotic nuclear beams at the SIS-FRS-ESR facility is summarized. New results on gross properties of exotic nuclei like binding energy, half-lives, and decay modes are presented. A brief outlook to future experiments is given.
Proton Inelastic Scattering onNi56in Inverse Kinematics
Inelastic proton scattering to the first excited ${2}^{+}$ state of the doubly magic $^{56}\mathrm{Ni}$ nucleus was investigated in inverse kinematics, using a secondary beam of radioactive $^{56}\mathrm{Ni}$ nuclei. At an incident energy of 101 MeV/nucleon, a value $B(E2,{0}^{+}\ensuremath{\rightarrow}{2}^{+})=600\ifmmode\pm\else\textpm\fi{}120 {e}^{2}$ ${\mathrm{fm}}^{4}$ was measured. This result completes the set of experimental data for the first excited ${2}^{+}$ states in the $1f\ensuremath{-}2p$ shell with a closed shell of neutrons or protons. These data are compared to recent shell-model calculations.
Mass mapping of a new area of neutron-deficient suburanium nuclides
Abstract The masses of 64 short-lived neutron-deficient nuclides covering the element range from tungsten to uranium have been obtained for the first time. They have been evaluated by combining directly measured masses from Schottky mass spectrometry with linked experimental Q-values in α-decay chains. Based on these new mass data we have determined the one-proton and two-proton drip-lines as well as the size of the “littoral shallow” of the sea of instability. No evidence of a Thomas–Ehrman shift has been found in the region of the investigated heavy nuclides. A peculiar behavior of two-proton separation energies has been observed in the lead region. The predictive power of various mass mo…
Study of the Unstable NucleusL10iin Stripping Reactions of the Radioactive ProjectilesB11eandL11i
Reactions of the halo systems Be-11 and Li-11 (at 460 and 280 MeV/nucleon) with a carbon target demonstrate that (n + Li-9) has an (unbound) l = 0 ground state very close to the threshold. The neutron halo of Li-11 has appreciable (1s(1/2))(2) and (0p(1/2))(2) components.
Population of nuclides with Z≥98 in multi-nucleon transfer reactions of 48Ca + 248Cm
The results for nuclei above curium, produced in multi-nucleon transfer reactions of 48Ca + 248Cm at the velocity filter SHIP of GSI Darmstadt, are presented. Spontaneous fission and α-activities have been used to study the population of nuclei with lifetimes ranging from few milliseconds to several days. We observed several, relatively neutron-rich isotopes with atomic numbers Z≥98; among them a weak 224 millisecond activity which we tentatively attributed to 260No. The measured cross-sections of the observed nuclei give hope that multi-nucleon transfer reactions are a way to reach new neutron-rich heavy and superheavy nuclei, which are not accessible in other reactions. We compare our res…
Fine structure in theαdecay ofPo188,192
The alpha decay of Po-188,Po-192 has been reexamined in order to probe the 0(+) states in the daughter nuclei Pb-184,Pb-188 that can be associated with coexisting spherical, oblate, and/or prolate ...
Halo excitations in fragmentation of He at 240 MeV/u on carbon and lead targets
Dissociation of a 240 MeV/u beam of He-6, incident on carbon and lead targets, has been studied in kinematically complete experiments to investigate low-lying excitation modes in the halo nucleus He-6. It is shown that alignment effects characterize the inelastic scattering and allow an unambiguous assignment of the spin of a narrow resonance observed in the excitation energy spectrum. The differential cross sections for the He-6 inelastic scattering on carbon and lead targets were deduced from the measured moments of the two neutrons and the a-particle. An analysis of these distributions shows that quadrupole and, possibly, monopole excitations characterize the hadronic interaction, while …
Development and test of iron-free quadrupole lenses with high magnetic flux densities
Abstract Iron-free magnetic quadrupole lenses have been developed for the focusing of energetic bunched heavy-ion beams. These devices are operated in a pulsed mode and provide very strong magnetic fields. A magnetic flux density of more than 14 T has been reached in a 100 mm long quadrupole with a 20 mm wide aperture, which corresponds to a magnetic flux density of ∼1400 T/m. The pulse duration of the applied electric current is approximately 300 μs with a flat top of several μs. The calculated and measured field properties of the quadrupoles are presented. In a first test experiment with a fast-extracted 650 MeV/u 197 Au 79+ beam (bunch length ∼500 ns) at GSI the focusing properties could…
Conversion electron and beta decay spectroscopy at SHIP
Abstract Novel methods for internal conversion electron and β -decay spectroscopy at the focal plane of a recoil separator are discussed. As an example the experimental data collected at the focal plane of the velocity filter SHIP (GSI, Darmstadt) are presented and compared with the results of the GEANT Monte Carlo simulations. It is shown that the simultaneous detection of conversion electrons, γ -rays and X-rays is possible, which significantly broadens the range of applications of this and similar systems.
Shape-changing particle decays ofBi185and structure of the lightest odd-mass Bi isotopes
Proton and alpha decay of the proton-rich nuclide Bi-185 has been restudied in more detail in the complete fusion reaction Nb-93(Mo-95, 3n)Bi-185 at the velocity filter SHIP. The observed decay pat ...
The Super-FRS Project at GSI
The GSI projectile fragment separator FRS has demonstrated with many pioneering experiments the research potential of in-flight separators at relativistic energies. Although the present facility has contributed much to the progress in the field of nuclear structure physics, major improvements are desirable in the future. The characteristics of the proposed next-generation facility at GSI, the Super-FRS, will be presented and compared to other projects. The Super-FRS is a large-acceptance superconducting fragment separator followed by different experimental branches including a combination with a new storage-cooler ring system. This system consists of a collector ring (CR) and a new experime…
Storage-ring experiments with exotic nuclei: from mass measurements to the future
Direct mass measurements with electron-cooled ions coasting in a heavy-ion storage ring allow the mapping of large areas of the nuclear chart, well suited to explore new regions and to investigate isospin effects as well as structure changes far-off stability. In this contribution first results will be discussed, experimental masses will be compared to theoretical predictions. A study of the isospin dependence of shell strength and pairing will be made.
Calculations of high-power production target and beamdump for the GSI future Super-FRS for a fast extraction scheme at the FAIR Facility
A superconducting fragment separator (Super-FRS) is being designed for the production and separation of radioactive isotopes at the future FAIR (Facility for Antiprotons and Ion Research) facility at Darmstadt. This paper discusses various aspects and requirements for the high-power production target that will be used in the Super-FRS experiments. The production target must survive over an extended period of time as it will be used during the course of many experiments. The specific power deposited by the high intensity beam that will be generated at the future FAIR facility will be high enough to destroy the target in most of the cases as a result of a single shot from the new heavy ion sy…
8He-6He: a comparative study of nuclear fragmentation reactions
19 pages, 3 tables, 6 figures.-- PACS nrs.: 27.20.+n; 24.70.+s; 25.06.-t.-- Available online Dec 4, 2000.
Status of the SHIPTRAP Project: A Capture and Storage Facility for Heavy Radionuclides from SHIP
The ion trap facility SHIPTRAP is being set up to deliver very clean and cool beams of singly-charged recoil ions produced at the SHIP velocity filter at GSI Darmstadt. SHIPTRAP consists of a gas cell for stopping and thermalizing high-energy recoil ions from SHIP, an rf ion guide for extraction of the ions from the gas cell, a linear rf trap for accumulation and bunching of the ions, and a Penning trap for isobaric purification. The progress in testing the rf ion guide is reported. A transmission of about 93(5)% was achieved.
He-8 - He-6: a comparative study of electromagnetic fragmentation reactions
14 pages, 1 table, 2 figures.-- PACS nrs.:27.20.+n; 24.70.+.-- Available online Oct 8, 2001.
Frontiers of Heavy - Ion Physics and Superheavy Elements
This contribution will focus on three topics of GSI nuclear structure research: super heavy elements, direct mass measurements in the storage ring, and the measurement of spallation cross section in reversed kinematics. The GSI project for an extended synchrotron facility will be outlined.
The dipole response of nuclei with large neutron excess
The dipole response of neutron-rich nuclei in the mass range from A = 10 to A = 22 and with mass to charge ratios of 2.5 to 2.8 has been invesitigated experimentally utilizing electromagnetic excitation in heavy-ion collisions at beam energies around 600 MeV/u.
SHE Research at GSI-Achievements and Plans
Experimental program of the Super-FRS Collaboration at FAIR and developments of related instrumentation
The physics program at the super-conducting fragment separator (Super-FRS) at FAIR, being operated in a multiple-stage, high-resolution spectrometer mode, is discussed. The Super-FRS will produce, separate and transport radioactive beams at high energies up to 1.5 AGeV, and it can be also used as a stand-alone experimental device together with ancillary detectors. Various combinations of the magnetic sections of the Super-FRS can be operated in dispersive, achromatic or dispersion-matched spectrometer ion-optical modes, which allow measurements of momentum distributions of secondary-reaction products with high resolution and precision. A number of unique experiments in atomic, nuclear and h…
New microsecond isomers in 189, 190Bi
New microsecond isomers in the neutron-deficient isotopes 189g, 190Bi have been identified after in-flight separation by the velocity filter SHIP. The evaporation residues were identified on the basis of delayed recoil-γ/X-ray, recoil-γ/X-ray-α and excitation function measurements. The systematics of the [ π1i 13/2]13/2+ excited states in the odd-mass Bi nuclei is discussed.
Experiments with stored exotic nuclei at relativistic energies
Abstract A review and recent progress are presented from experiments on masses and lifetimes of bare and few-electron exotic nuclei at GSI. Relativistic rare isotopes produced via projectile fragmentation and fission were separated in flight by the fragment separator FRS and injected into the storage ring ESR. This worldwide unique experimental method gives access to all fragments with half-lives down to the microsecond range. The great research potential is demonstrated by the discovery of new isotopes along with simultaneous mass and lifetime measurements. Single particle decay measurements and the continuous recording of both stored mother and daughter nuclei open up a new era for nuclea…
Attempts to Produce Superheavy Elements by Fusion ofCa48withCm248in the Bombarding Energy Range of 4.5-5.2 MeV/u
A search for superheavy elements was made in bombardments of $^{248}\mathrm{Cm}$ with $^{48}\mathrm{Ca}$ ions performed at projectile energies close to the interaction barrier in order to keep the excitation energy of the compound nucleus $Z=116$, $A=296$ as low as possible. No evidence for superheavy nuclei was obtained in a half-life region from 1 \ensuremath{\mu}s to 10 yr with a production cross section greater than ${10}^{\ensuremath{-}34}$ to ${10}^{\ensuremath{-}35}$ ${\mathrm{cm}}^{2}$.
Ion-optical layout of a powerful next-generation pre-separator for in-flight separation of relativistic rare isotopes
Abstract Rare isotope beams can be efficiently produced at relativistic energies via projectile fragmentation and projectile fission. Magnetic rigidity analysis in combination with atomic energy loss ( Bρ –Δ E – Bρ method) in profiled matter placed at dispersive focal planes represents the tool for spatial separation in flight. The next-generation in-flight separators at high energies will consist of multiple degrader stages to provide intense monoisotopic fragment beams of all elements up to uranium. The pre-separator layout with the first degrader system holds many technical challenges, e.g. to handle the high-power primary beams characterized by a large range in time structure, from a DC…
Quasi-free scattering with 6,8He beams
Abstract This paper presents the results of experimental investigations of ( p , p n ) , ( p , p α ) and ( p , p 6 He) reactions with relativistic 6 He and 8 He beams impinging on a hydrogen target. Information on the structure of extremely neutron-rich nuclei was obtained by using the unique characteristic of quasi-free scattering processes and inverse kinematics. For the first time, momentum distributions of complex clusters inside 6 He and 8 He were measured. Spectroscopic factors for valence neutrons, α - and 6 He clusters were deduced from the experimental data. They demonstrate that the filling of the p 1 2 shell is the essential feature of the 8 He structure. It is shown that the 8 H…
Longitudinal and transverse momentum distributions of 9Li fragments from break-up of 11Li
7 pages, 3 figures, 1 table.
Experiments with Exotic Atoms and Exotic Nuclei at GSI, Recent Developments and Future Prospects
Results and new developments with exotic atoms and exotic nuclei are presented from recent experiments at GSI. The proposed European inflight facility at GSI will open up new fields of outstanding research and will simultaneously access unknown regions of nuclei with new properties. A new generation of precision experiments will be performed with stored exotic nuclei, whereby nuclear reactions with an internal target and electron scattering in a small electron-ion collider will be a great challenge.
Schottky mass measurements of stored and cooled neutron-deficient projectile fragments in the element range of 57≤Z≤84
Abstract A novel method for direct, high precision mass measurements of relativistic exotic nuclei has been successfully applied in the storage ring ESR at GSI. The nuclei of interest were produced by projectile fragmentation of 930 MeV / u bismuth ions, separated in-flight by the fragment separator FRS, stored and cooled in the ESR. The mass values have been deduced from the revolution frequencies of the coasting cooled ions. We have measured 104 new mass values with a precision of about 100 keV and a resolving power of 3.5×10 5 for the neutron-deficient isotopes of the elements 57≤Z≤84 . This paper presents the experimental method, the mass evaluation and a table of the experimental mass …