0000000000030853

AUTHOR

Werner Lauth

showing 49 related works from this author

Experimental investigations of backward transition radiation characteristics in extreme ultraviolet region

2011

ABSTRACT This report summarizes the results of an experiment dedicated to the observation of backward transition radia-tion in the EUV spectral region. This radiation was ge nerated by an 855MeV electron beam at a molybdenumtarget. The radiation characteristics in the EUV region are compared to those in the optical region. It wasshown that the radiation measured in the EUV region was more intense than theoretically predicted. As aresult the EUV radiation yield seems to be suci ent for standard beam pro“le diagnostics.Keywords: EUV, Transition radiation, Beam diagnostics 1. INTRODUCTION Transverse pro“le diagnostics in mo dern electron linear accelerators as F ELs or injector linacs is mainl…

PhysicsOpticsTransition radiationbusiness.industryExtreme ultraviolet lithographyExtreme ultravioletElectronRadiationbusinessParticle beamBeam (structure)Linear particle acceleratorSPIE Proceedings
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The PANDA Barrel DIRC detector

2014

Abstract The PANDA experiment at the new Facility for Antiproton and Ion Research in Europe (FAIR) at GSI, Darmstadt, will study fundamental questions of hadron physics and QCD using high-intensity cooled antiproton beams with momenta between 1.5 and 15 GeV/c. Efficient Particle Identification for a wide momentum range and the full solid angle is required for reconstructing the various physics channels of the PANDA program. Hadronic Particle Identification in the barrel region of the detector will be provided by a DIRC counter. The design is based on the successful BABAR DIRC with important improvements, such as focusing optics and fast photon timing. Several of these improvements, includin…

PhysicsNuclear and High Energy PhysicsParticle physicsPhotonLarge Hadron ColliderPhysics::Instrumentation and DetectorsHadronDetectorParticle identificationNuclear physicsConceptual designAntiprotonPhysics::Accelerator PhysicsFacility for Antiproton and Ion ResearchHigh Energy Physics::ExperimentNuclear ExperimentInstrumentationNuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment
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Characterization and Tuning of Ultra High Gradient Permanent Magnet Quadrupoles

2009

The application of quadrupole devices with high field gradients and small apertures requires precise control over higher order multipole field components. We present a new scheme for performance control and tuning, which allows the illumination of most of the quadrupole device aperture because of the reduction of higher order field components. Consequently, the size of the aperture can be minimized to match the beam size achieving field gradients of up to $500\text{ }\text{ }\mathrm{T}\text{ }{\mathrm{m}}^{\ensuremath{-}1}$ at good imaging quality. The characterization method based on a Hall probe measurement and a Fourier analysis was confirmed using the high quality electron beam at the M…

Accelerator Physics (physics.acc-ph)electron beamNuclear and High Energy PhysicsPhysics - Instrumentation and DetectorscompactmagneticlensPhysics and Astronomy (miscellaneous)Field (physics)AperturemultipoleFOS: Physical sciencespermanenthalbachx-felNuclear magnetic resonancetuningquadrupolelcsh:Nuclear and particle physics. Atomic energy. RadioactivityQuadrupole magnetMicrotronPhysicsOrder (ring theory)Surfaces and InterfacesInstrumentation and Detectors (physics.ins-det)beam focusingComputational physicsMagnetQuadrupolelcsh:QC770-798Physics::Accelerator PhysicsPhysics - Accelerator PhysicsMultipole expansion
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A compact apparatus for mass selective resonance ionization spectroscopy in a buffer gas cell

1997

Abstract An ultra-sensitive laser spectroscopic method for the investigation of transuranium nuclides has been developed based on resonance ionization in an argon buffer gas cell. This method has been combined with ion-guide extraction and mass selective direct detection of the resonantly ionized atoms. Using argon as a buffer gas, recoils of fusion reactions can be thermalized even at low pressure. The differential pumping system consists of only one roots pump and two turbo molecular pumps. The set-up has been tested with 243 Am evaporated from a filament located inside the optical gas cell. Resonance ionization is performed using a two-step excitation with an excimer-dye-laser combinatio…

Nuclear and High Energy PhysicsArgonBuffer gasAnalytical chemistrychemistry.chemical_elementMass spectrometryIon sourceAtmospheric-pressure laser ionizationchemistryIonizationAtomic physicsInstrumentationQuadrupole mass analyzerElectron ionizationNuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
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Characterization of SiPM properties at liquid nitrogen temperature

2016

SiPM operation at cryogenic temperatures fails for many common devices. A particular type with deep channels in the silicon substrate instead of quenching resistors was thoroughly characterized from room temperature down to liquid nitrogen temperature by illuminating it with low light levels. The devices were mounted in vacuum with the temperature stabilized to allow long-term operation. SiPM signals from a LED pulser were acquired with single-pixel resolution. Generalized fits to the charge collection spectra were used to extract properties like single-pixel gain, inter-pixel variation, breakdown voltage, and photon detection efficiency. With these measurements a deeper investigation of th…

Materials scienceSiliconPhysics::Instrumentation and Detectors010308 nuclear & particles physicsbusiness.industrychemistry.chemical_elementCryogenicsLiquid nitrogen01 natural sciencesSpectral linelaw.inventionSilicon photomultiplierchemistrylaw0103 physical sciencesOptoelectronicsBreakdown voltagePhotonicsResistorbusiness2016 IEEE Nuclear Science Symposium, Medical Imaging Conference and Room-Temperature Semiconductor Detector Workshop (NSS/MIC/RTSD)
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Channeling and Radiation of Electrons in Silicon Single Crystals and Si1−xGexCrystalline Undulators

2013

The phenomenon of channeling and the basic features of channeling radiation emission are introduced in a pedestrian way. Both, radiation spectra as well as dechanneling length measurements at electron beam energies between 195 and 855 MeV feature quantum state phenomena for the (110) planar potential of the silicon single crystals. Radiation from a crystalline undulator, produced at the Aarhus University (UAAR), has been investigated at the Mainz Microtron electron accelerator facility MAMI. The 4-period epitaxially grown strained layer Si1−xGex undulator had a period length λu = 9.9 μm. At a beam energy of 375 MeV a broad excess yield around the theoretically expected photon energy of 0.13…

PhysicsHistorySiliconchemistry.chemical_elementParticle acceleratorElectronPhoton energyRadiationUndulatorComputer Science ApplicationsEducationlaw.inventionchemistrylawCathode rayPhysics::Accelerator PhysicsAtomic physicsNuclear ExperimentMicrotronJournal of Physics: Conference Series
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Backward transition radiation in the extreme ultraviolet region as a tool for the transverse beam profile diagnostic

2014

The present article summarizes the results of two experiments which were performed to study the radiation properties of backward transition radiation (BTR) in the extreme ultraviolet (EUV) region. This wavelength region is of particular interest for transverse beam profile imaging, because the spatial resolution is improved as a result of the reduced contribution in the imaging process of the fundamental diffraction limit. In addition, the influence of coherent effects in the transition radiation emission process, which have been observed in the visible region, might be mitigated. The first experiment, dedicated to the investigation of the BTR angular characteristics, indicates that the rad…

DiffractionPhysicsNuclear and High Energy PhysicsPhysics and Astronomy (miscellaneous)business.industryExtreme ultraviolet lithographySurfaces and InterfacesRadiationRadiation propertiesWavelengthOpticsTransition radiationExtreme ultravioletlcsh:QC770-798ddc:530lcsh:Nuclear and particle physics. Atomic energy. RadioactivitybusinessBeam (structure)Physical Review Special Topics. Accelerators and Beams
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Experimental realization of a new type of crystalline undulator.

2014

A new scheme of making crystalline undulators was recently proposed and investigated theoretically by Andriy Kostyuk, concluding that a new type of crystalline undulator would be not only viable, but better than the previous scheme. This article describes the first experimental measurement of such a crystalline undulator, produced by using Si(1-x)Ge(x)-graded composition and measured at the Mainzer Microtron facility at beam energies of 600 and 855 MeV. We also present theoretical models developed to compare with the experimental data.

OpticsMaterials sciencebusiness.industryTheoretical modelsGeneral Physics and AstronomyType (model theory)UndulatorbusinessMicrotronRealization (systems)Beam (structure)Physical review letters
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Probing Sizes and Shapes of Nobelium Isotopes by Laser Spectroscopy

2018

Until recently, ground-state nuclear moments of the heaviest nuclei could only be inferred from nuclear spectroscopy, where model assumptions are required. Laser spectroscopy in combination with modern atomic structure calculations is now able to probe these moments directly, in a comprehensive and nuclear-model-independent way. Here we report on unique access to the differential mean-square charge radii of ^{252,253,254}No, and therefore to changes in nuclear size and shape. State-of-the-art nuclear density functional calculations describe well the changes in nuclear charge radii in the region of the heavy actinides, indicating an appreciable central depression in the deformed proton densi…

IN-BEAMNuclear TheoryGeneral Physics and Astronomychemistry.chemical_element[PHYS.NEXP]Physics [physics]/Nuclear Experiment [nucl-ex]DROPLET-MODEL01 natural sciencesEffective nuclear chargeNO-2540103 physical sciencesNeutronSUPERHEAVY ELEMENTS010306 general physicsSpectroscopyMASSESNuclear ExperimentHyperfine structurePhysicsMagnetic momentNUCLEI010308 nuclear & particles physicsPRODUCTSchemistryQuadrupoleUPDATENobeliumAtomic physicsSHIPNuclear density
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Spectral distribution and Coulomb correction for nuclear bremsstrahlung induced by heavy targets

2021

Abstract Bremsstrahlung spectra below 250 MeV have been measured colliding 500 MeV–electrons with Cu, Ag, and Au targets. The experimental intensity ratios relative to Cu are well described by an accurate analytical high-energy theory, which accounts both for Coulomb distortion and screening. This represents the first experimental verification of the discovery by Bethe-Maximon that leading-order quantum mechanical calculations, equivalent to quasiclassical approximations, become exact at high energies and small angles. It also shows that radiative QED effects play a minor role in the covered part of the spectral distribution within the accuracy (1.6%) of the present measurements.

PhysicsQuantum electrodynamicsNuclear and High Energy PhysicsSpectral power distributionMECÂNICA QUÂNTICAHigher-order theory010308 nuclear & particles physicsBremsstrahlungBremsstrahlungIntensity ratio01 natural sciencesSpectral linelcsh:QC1-999Nuclear physicsDistortion0103 physical sciencesCoulombRadiative transfer010306 general physicsQuantumlcsh:PhysicsCoulomb correctionPhoton spectra
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First Observation of Atomic Levels for the Element Fermium (Z=100)

2003

The atomic level structure of the element fermium was investigated for the first time using a sample of $2.7\ifmmode\times\else\texttimes\fi{}{10}^{10}$ atoms of the isotope $^{255}\mathrm{F}\mathrm{m}$ with a half-life of 20.1 h. The atoms were evaporated from a filament and stored in the argon buffer gas of an optical cell. Atomic levels were sought by the method of resonance ionization spectroscopy using an excimer-dye-laser combination. Two atomic levels were found at wave numbers $(25\text{ }099.8\ifmmode\pm\else\textpm\fi{}0.2)$ and $(25\text{ }111.8\ifmmode\pm\else\textpm\fi{}0.2)\text{ }\text{ }{\mathrm{c}\mathrm{m}}^{\ensuremath{-}1}$. Partial transition rates to the $5{f}^{12}7{s}…

PhysicschemistryFermiumResonance ionizationSaturation (graph theory)General Physics and Astronomychemistry.chemical_elementAtomic physicsGround stateSpectroscopyPhysical Review Letters
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Radiation detected resonance ionization spectroscopy on208Tl and242fAm

1993

An ultra-sensitive laser spectroscopic method has been developed for the hyperfine spectroscopy of short-lived isotopes far off stability produced by heavy ion induced nuclear reactions at very weak intensity (> 1/s). It is based on resonance ionization spectroscopy in a buffer gas cell with radiation detection of the ionization process (RADRIS). As a first on-line application of RADRIS optical spectroscopy at242fAm fission isomers is in progress at the low target production rate of 10/s. The resonance ionization has been performed in two steps utilizing an excimer dye laser combination with a repetition rate of 300 Hz. The first resonant step proceeds through terms which correspond to wave…

Nuclear and High Energy PhysicsDye laserExcimer laserChemistrymedicine.medical_treatmentAnalytical chemistryResonanceCondensed Matter PhysicsAtomic and Molecular Physics and OpticsIon sourceAtmospheric-pressure laser ionizationIonizationmedicinePhysical and Theoretical ChemistryAtomic physicsSpectroscopyAmbient ionizationHyperfine Interactions
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Modeling and Characterization of SiPM Parameters at Temperatures between 95 K and 300 K

2017

The modeling and characterization of silicon photomultipliers (SiPMs) in a wide temperature range from 95 K to 300 K is presented. The devices under study had the distinctive feature of forward-biased p-n junctions situated under each pixel as active quenching resistors making them particularly appropriate to be operated at cryogenic temperatures. The voltage drop across the diode in a forward direction was measured for a series of injected currents in this temperature range. It was observed that the characteristics of different SiPM types influence the temperature dependence of the reverse saturation current. The devices were further characterized by low-level light-pulse measurements. The…

QuenchingNuclear and High Energy PhysicsMaterials sciencePhysics::Instrumentation and Detectors010308 nuclear & particles physicsbusiness.industryCryogenicsAtmospheric temperature range01 natural sciences030218 nuclear medicine & medical imaginglaw.invention03 medical and health sciences0302 clinical medicineSilicon photomultiplierNuclear Energy and EngineeringlawSaturation current0103 physical sciencesOptoelectronicsElectrical and Electronic EngineeringResistorbusinessVoltage dropDiodeIEEE Transactions on Nuclear Science
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Forward diffracted parametric X radiation from a silicon single crystal

2005

Experiments were performed with the 855 MeV electron beam of the Mainz Microtron MAMI which focused on still open questions in the X-ray emission process upon traversal of ultra relativistic electrons through single crystals. To elucidate the quest of kinematical versus dynamical production of PXR the radiation from silicon single crystal targets, emitted close to the electron direction, has been studied. The observed interference structures show that PXR is produced in a dynamical process.

PhysicsDiffractionNuclear and High Energy PhysicsSiliconbusiness.industryAstrophysics::High Energy Astrophysical Phenomenachemistry.chemical_elementElectronRadiationOpticschemistryInterference (communication)Cathode rayAtomic physicsNuclear ExperimentbusinessInstrumentationMicrotronSingle crystalNuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
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First Determination of the Ionization Potential of Actinium and First Observation of Optical Transitions in Ferminm

2002

For the determination of the first ionization potential of actinium, 227Ac was electrodeposited on a Ta backing and covered with ~1 μm Zr. From this filament, Ac atoms were evaporated at ≥ 1250 °C. By resonant excitation with UV light of 388.67 nm and subsequent excitation with light of ca. 568 nm, Ac was ionized in an external electrical field. By determining the ionization thresholds as a function of the electrical field strength and by extrapolation to zero field strength, the first ionization potential of 43398(3) cm−1 = 5.3807(3) eV was measured.About 1 ng of 255Fm, half life 20.1 h, was prepared at ORNL by milking from 255Es produced in the High Flux Isotope Reactor and shipped to Mai…

Nuclear and High Energy PhysicsChemistryBuffer gasAnalytical chemistryThermal ionizationchemistry.chemical_elementIonActiniumNuclear Energy and EngineeringExcited stateIonizationAtomic physicsIonization energyExcitationJournal of Nuclear Science and Technology
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Resonance ionization spectroscopy of fermium (Z=100)

2003

Laser spectroscopy has been applied for the first time to measure resonant transition frequencies of fermium (Zs 100). A number of 2.7=10 atoms was electrodeposited on a Ta filament and covered with a 1 mm Ti layer. Fm 10

ChemistryFermiumBuffer gasAnalytical chemistrychemistry.chemical_elementPhotoionizationActinideAtomic and Molecular Physics and OpticsAnalytical ChemistryProtein filamentIonizationAtomic physicsSpectroscopyAbsorption (electromagnetic radiation)InstrumentationSpectroscopySpectrochimica Acta Part B: Atomic Spectroscopy
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The experimental setup of the Interaction in Crystals for Emission of RADiation collaboration at Mainzer Mikrotron: Design, commissioning, and tests

2015

Silicon/germanium flat/bent crystals are thin devices able to efficiently deflect charged particle GeV-energy beams up to a few hundreds of μrad; moreover, high intensity photons can be efficiently produced in the so-called Multi-Volume Reflection (MVR) and Multiple Volume Reflections in One Crystal (MVROC) conditions. In the last years, the research interest in this field has moved to the dynamic studies of light negative leptons in the low energy range: the possibility to deflect negative particles and to produce high intensity γ sources via the coherent interactions with crystals in the sub-GeV energy range has been proved by the ICE-RAD (Interaction in Crystals for Emission of RADiation…

PhotonPhysics::Instrumentation and DetectorsCrystals characterizationsBENT CRYSTALSCoherent interaction; Crystals characterizations; High intensity gamma sources;ScintillatorCoherent interactionVOLUME REFLECTION; CHARGED-PARTICLES; BENT CRYSTALS; SILICON; MICROTRONNOOpticsSILICONInstrumentationPhysicsRange (particle radiation)High intensity gamma sourcesbusiness.industryVOLUME REFLECTIONCharged particleCHARGED-PARTICLESBeamlineGoniometerMICROTRONScintillation counterPhysics::Accelerator PhysicsProfilometerbusiness
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INVESTIGATION OF FAR-INFRARED SMITH-PURCELL RADIATION AT THE 3.41 MEV ELECTRON INJECTOR LINAC OF THE MAINZ MICROTRON MAMI

2006

PhysicsNuclear physicsFar infraredlawCathode rayInjectorElectronRadiationMicrotronLinear particle acceleratorlaw.invention
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Resonance ionization spectroscopy in a buffer gas cell with radioactive decay detection, demonstrated usingTl208

1992

An ultrasensitive laser spectroscopic method has been developed to perform hyperfine spectroscopy of heavy-ion-induced reaction products. It is based on resonance ionization in a buffer gas cell combined with radioactive decay detection. The feasibility has been demonstrated using the \ensuremath{\beta}-active ${\mathrm{isotope}}^{208}$ Tl. A sensitivity of 1.3\ifmmode\times\else\texttimes\fi{}${10}^{\mathrm{\ensuremath{-}}3}$ of the two-step resonance-ionization process via the n=17 Rydberg level has been determined, utilizing a pulsed excimer-dye-laser combination. The previously unknown nuclear magnetic moment \ensuremath{\mu}${(}^{208}$Tl) = 0.292(13)${\mathrm{\ensuremath{\mu}}}_{\mathi…

PhysicsMagnetic momentExcited stateNuclear magnetic momentGeneral Physics and AstronomyResonanceSensitivity (control systems)Atomic physicsHyperfine structureNuclear magnetonRadioactive decayPhysical Review Letters
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Enhancement of Bremsstrahlung Radiation Generated by Electron Beam Interaction in an Axially-Oriented Scintillator Crystal (Poster)

2019

Since their discovery, scintillator materials have played an important role in nuclear and particle physics, as well as in medical and industrial imaging. [...]

Physics::Computational PhysicsMaterials sciencebusiness.industryPhysics::Instrumentation and DetectorsBremsstrahlunglcsh:AScintillatorComputer Science::Numerical AnalysisIndustrial imagingCrystalOpticsn/aCathode raylcsh:General WorksbusinessAxial symmetryProceedings
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Radiation emission at channeling of electrons in a strained layer undulator crystal

2013

Abstract Experiments have been performed at the Mainz Microtron MAMI to explore the radiation emission spectra from a crystalline undulator at electron beam energies of 270 and 855 MeV. The epitaxially grown graded composition strained layer Si 1 - x Ge x undulator had 4-period with a period length λ u = 9.9 μ m . Spectra taken at the beam energy of 270 MeV at channeling in the undulating (110) planes exhibit a broad excess yield around the theoretically expected photon energies of 0.069 MeV, as compared with a flat silicon reference crystal. Model calculations on the basis of synchrotron-like radiation emission from finite single arc elements, taking into account also coherence effects, su…

010302 applied physicsPhysicsNuclear and High Energy PhysicsPhotonSiliconchemistry.chemical_elementElectronUndulator01 natural sciencesSpectral lineCrystalchemistry0103 physical sciencesCathode rayPhysics::Accelerator PhysicsAtomic physicsNuclear Experiment010306 general physicsInstrumentationMicrotronNuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
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Performance of sensl C-Series SiPM with high photoelectron resolution at cryogenic temperatures

2016

The C-Series of silicon photomultipliers (SiPM) from SensL provides devices with a fast response and high performance at low cost. The device's ability to detect light at temperatures of liquid nitrogen (77K) and liquid helium (4 K) with high photoelectron resolution was demonstrated. Results include relative photon detection efficiency (PDE), gain, microcell capacitance, and cross-talk probability at different over-voltages, both at room and at cryogenic temperatures. At 77K the SiPM demonstrated significantly improved operating characteristics while at 4K the observed increase in break-down voltage, the reduction of PDE by a factor of 2-3, and the extensively dropped microcell capacitance…

Materials sciencebusiness.industryLiquid heliumchemistry.chemical_elementLiquid nitrogenCapacitancelaw.inventionSilicon photomultiplierchemistrylawElectronic engineeringOptoelectronicsMicrocellPhotonicsbusinessHeliumVoltage2016 IEEE Nuclear Science Symposium, Medical Imaging Conference and Room-Temperature Semiconductor Detector Workshop (NSS/MIC/RTSD)
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<title>Forward diffracted parametric X radiation from a thick Tungsten single crystal at 855 MeV electron energy</title>

2007

Features of forward diffracted Parametric X-Radiation (PXR) were investigated at experiments with the 855 MeV electron beam of the Mainz Microtron MAMI employing a 410 micrometer thick tungsten single crystal. Virtual photons from the electron field are diffracted by the (10-1) plane at a Bragg angle of 3.977 degree. Forward emitted radiation was analyzed at an energy of 40 keV with the (111) lattice planes of a flat silicon single crystal in Bragg geometry. Clear peak structures were observed in an angular scan of the tungsten single crystal. The results were analyzed with a model which describes forward diffracted PXR under real experimental conditions. The experiments show that forward d…

DiffractionMaterials sciencebusiness.industryPhysics::Opticschemistry.chemical_elementBragg's lawTungstenRadiationField electron emissionOpticschemistryCathode raybusinessSingle crystalMicrotronSPIE Proceedings
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Developments for resonance ionization laser spectroscopy of the heaviest elements at SHIP

2016

Abstract The experimental determination of atomic levels and the first ionization potential of the heaviest elements ( Z ⩾ 100 ) is key to challenge theoretical predictions and to reveal changes in the atomic shell structure. These elements are only artificially produced in complete-fusion evaporation reactions at on-line facilities such as the GSI in Darmstadt at a rate of, at most, a few atoms per second. Hence, highly sensitive spectroscopic methods are required. Laser spectroscopy is one of the most powerful and valuable tools to investigate atomic properties. In combination with a buffer-gas filled stopping cell, the Radiation Detected Resonance Ionization Spectroscopy (RADRIS) techniq…

YtterbiumNuclear and High Energy Physics010308 nuclear & particles physicschemistry.chemical_elementInstrumental chemistry01 natural sciencesAtmospheric-pressure laser ionizationchemistryExcited state0103 physical sciencesPhysics::Atomic PhysicsNobeliumLaser-induced breakdown spectroscopyIonization energyAtomic physics010306 general physicsSpectroscopyInstrumentationNuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
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Development of an Endcap DIRC for PANDA

2014

Abstract The aim of this research is to develop a planar DIRC detector showing advantages and performance similar to a classical, barrel shaped DIRC, but at smaller polar angles which cannot be accessed using a cylindrical geometry. The device will complement the PANDA Barrel DIRC by covering polar angles from 5° to 22°. The envisaged π /K-separation is ≥ 3 σ up to 4 GeV/c. A major challenge is the adaption of the device to the PANDA environment including a magnetic field of ~1–2 T, high rates and radiation, limited space for optics and sensors as well as the lack of a common first-level trigger. This paper discusses a detector design which forms a compromise between these constraints and a…

PhysicsHigh rateNuclear and High Energy PhysicsPhysics::Instrumentation and Detectorsbusiness.industryDetectorBarrel (horology)Reconstruction methodParticle identificationOpticsPlanarHigh Energy Physics::ExperimentDevelopment (differential geometry)businessInstrumentationCherenkov radiationNuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment
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Fission fragment anisotropy for the 242mAm fission isomer by spin exchange pumping with polarized rubidium vapour

1992

Abstract The foundations of an experiment have been worked out with which, in principle, the spin, hyperfine constants and the isomer shift of the 14 ms fission isomer 242mAm can be measured. Such an experiment would be based on the fission fragment anisotropy signal which has actually been observed in this work after spin exchange pumping with polarized rubidium vapour in an optical buffer gas cell. A decrease of the count rate of (12±4)% has been measured at 90% with respect to the quantization axis. From this result it is concluded that the nuclear spin of the 242mAm fission isomer must be larger than 1. The low-energy fission isomers originating from the 242Pu(d, 2n)242mAm reaction have…

Nuclear reactionNuclear and High Energy PhysicsCluster decayFissionChemistrychemistry.chemical_elementAmericiumRubidiumNuclear physicsPlutonium-242Physics::Atomic and Molecular ClustersAtomic physicsNuclear ExperimentSpin (physics)InstrumentationHyperfine structureNuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
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Direct Measurement of Focusing Fields in Active Plasma Lenses

2018

Physical review accelerators and beams 21(12), 122801 (2018). doi:10.1103/PhysRevAccelBeams.21.122801

Accelerator Physics (physics.acc-ph)Nuclear and High Energy PhysicsPhysics and Astronomy (miscellaneous)Field (physics)FOS: Physical sciences01 natural sciences530law.inventionOpticslaw0103 physical sciencesddc:530Thermal emittancelcsh:Nuclear and particle physics. Atomic energy. Radioactivity010306 general physicsphysics.acc-phPhysics010308 nuclear & particles physicsbusiness.industrySurfaces and InterfacesPlasmaNuclear & Particles PhysicsLens (optics)Physics::Space PhysicsPhysical SciencesCathode raylcsh:QC770-798Physics::Accelerator PhysicsPhysics - Accelerator PhysicsBeam emittancebusinessCharged particle beamBeam (structure)
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Prospects for laser spectroscopy, ion chemistry and mobility measurements of superheavy elements in buffer-gas traps

2015

Abstract Laser spectroscopic methods are reviewed which are of potential interest for the investigation of atomic and ionic level structures of superheavy elements. The latter are defined here as the trans-fermium elements with Z > 100 for which no experimental atomic or ionic level structure information is known so far, and which cannot be bred in high flux nuclear power reactors via successive neutron capture. The principles of suitable laser spectroscopic methods are described, and illustrated by examples of real experiments. The addressed methods include single-ion spectroscopy in Paul traps, laser-induced fluorescence spectroscopy (LIF), radiation-detected optical pumping (RADOP), radi…

PhysicsNuclear and High Energy PhysicsBuffer gasIonic bondingElectronic structureLaserFluorescence spectroscopylaw.inventionIonNeutron capturelawPhysics::Atomic PhysicsAtomic physicsSpectroscopyNuclear Physics A
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Atom-at-a-time laser resonance ionization spectroscopy of nobelium

2016

Resonance ionization spectroscopy of nobelium (atomic number 102) reveals its ground-state transition and an upper limit for its ionization potential, paving the way to characterizing even heavier elements via optical spectroscopy. Characterizing the heaviest elements in the periodic table is a gruelling task because they are radioactive, exist only for split seconds at a time and need to be artificially produced in sufficient quantities by complicated procedures. The heaviest element that has been characterized by optical spectroscopy is fermium, which has an atomic number of 100. Mustapha Laatiaoui et al. extend the methods used for fermium to perform optical spectroscopy on nobelium (ato…

PhysicsMultidisciplinary010308 nuclear & particles physicsFermiumchemistry.chemical_element[PHYS.NEXP]Physics [physics]/Nuclear Experiment [nucl-ex]7. Clean energy01 natural scienceschemistry13. Climate actionIonization0103 physical sciencesAtomAtomic numberNobeliumPhysics::Atomic PhysicsAtomic physics010306 general physicsSpectroscopyRelativistic quantum chemistryLawrenciumNature
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Precision Measurement of the First Ionization Potential of Nobelium

2018

One of the most important atomic properties governing an element's chemical behavior is the energy required to remove its least-bound electron, referred to as the first ionization potential. For the heaviest elements, this fundamental quantity is strongly influenced by relativistic effects which lead to unique chemical properties. Laser spectroscopy on an atom-at-a-time scale was developed and applied to probe the optical spectrum of neutral nobelium near the ionization threshold. The first ionization potential of nobelium is determined here with a very high precision from the convergence of measured Rydberg series to be 6.626 21±0.000 05  eV. This work provides a stringent benchmark for st…

ENERGIESGeneral Physics and Astronomychemistry.chemical_elementElectron[PHYS.NEXP]Physics [physics]/Nuclear Experiment [nucl-ex]01 natural sciences7. Clean energysymbols.namesakeIonizationEQUAL-TO 1040103 physical sciencesLAWRENCIUMBUFFER GASPhysics::Atomic PhysicsSUPERHEAVY ELEMENTSLASER SPECTROSCOPY010306 general physicsSpectroscopyPhysicsNEUTRAL YTTERBIUM010308 nuclear & particles physicsHEAVIEST ELEMENTSchemistryRydberg formulasymbolsEXCITED-LEVELSNobeliumACTINIDESIonization energyAtomic physicsRelativistic quantum chemistryLawrencium
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Miniature magnetic devices for laser-based, table-top free-electron lasers

2007

Truly table-top sized radiation sources based on compact laser-plasma accelerators require compact and strong focusing devices and efficient short-period undulators. Complementing our recent theoretical work on the feasibility of a table-top FEL, we here present the design and successful experimental characterizations of a 5 mm period length undulator and miniature quadrupole magnets with field gradients of the order of $500\text{ }\text{ }\mathrm{T}/\mathrm{m}$.

Free electron modelNuclear and High Energy PhysicsPhysics and Astronomy (miscellaneous)Field (physics)41.75.JvRadiationlaw.inventionOpticslaw41.60.Crlcsh:Nuclear and particle physics. Atomic energy. RadioactivityQuadrupole magnetPhysicsFELbusiness.industryOrder (ring theory)magnet designSurfaces and InterfacesUndulatorLaserpacs:41.85.Lc52.38.KdOptoelectronicsPhysics::Accelerator Physicslcsh:QC770-798Strong focusingbusinessPhysical Review Special Topics. Accelerators and Beams
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Prospects of Ion Chemical Reactions with Heavy Elements in the Gas Phase

2001

Heavy element chemistry is related to the fundamental interest that lies in exploring the upper limits of the periodic table. Chemical properties of the heaviest elements have already been studied at single atoms in aqueous solutions and in the gas phase up to an atomic number Z = 107. These techniques allow to study nuclides with half lives as short as about 1 s. Next generation chemistry experiments could be envisaged with an ion trap technique already developed for stable isotopes. At very low production rates in the order of 1 per 100 s and/or half lives as short as about 10 ms, the ion-molecule reactions can be studied in a buffer gas cell, in which the heavy elements are stopped and t…

Aqueous solutionChemistryStable isotope ratioBuffer gasNuclideAtomic numberIon trapAtomic physicsChemical reactionIon
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Planar channeling experiments with electrons at the 855MeV Mainz Microtron MAMI

2008

Abstract Planar channeling has been studied for silicon single crystals at a beam energy of 855 MeV at the Mainz Microtron MAMI. Complex channeling patterns were observed from which the crystal orientation can unambiguously be determined. Photon spectra at (1 0 0), (1 1 0) and (1 1 1) planar channeling were recorded with a 10″ × 10″ NaI detector. The planar (1 1 0) channeling process has been studied as function of the crystal thickness in the range between 7.9 and 270 μm from which a dechanneling length of 18.0 μm and the thickness dependent rechanneling lengths were deduced, employing solutions of the Fokker–Planck equation. A signal derived from high energy bremsstrahlung exhibits a char…

PhysicsNuclear and High Energy PhysicsRange (particle radiation)SiliconBremsstrahlungchemistry.chemical_elementElectronMonocrystalline siliconCrystalPlanarchemistryAtomic physicsInstrumentationMicrotronNuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
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Isotope Shift Measurements for Superdeformed Fission Isomeric States

1998

Optical isotope shift measurements have been performed for the ${}^{240,242}{\mathrm{Am}}^{f}$ fission isomers with low target production rates of $10{\mathrm{s}}^{\ensuremath{-}1}$ employing resonance ionization spectroscopy in a buffer gas cell. Isotope shift ratios ${\mathrm{IS}}^{240f,241}/{\mathrm{IS}}^{243,241}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}39.2(8)$ and ${\mathrm{IS}}^{242f,241}/{\mathrm{IS}}^{243,241}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}41.4(8)$ have been measured at the 500.02 nm transition. A difference in the nuclear mean charge radii $\ensuremath{\delta}〈{r}^{2}{〉}_{\mathrm{opt}}^{242f,241}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}5.34(2…

PhysicsIsotopeFissionResonance ionizationQuadrupoleGeneral Physics and AstronomyCharge (physics)Production (computer science)Atomic physicsPhysical Review Letters
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Resonant transition radiation in the X-ray region from a low emittance 855 MeV electron beam

1994

The interference of transition radiation coherently produced from a periodic stack of four polyimide foils of 7.2 μm thickness and a separation of 162 μm was investigated. This stack has been brought into the low emittance (3 π nm rad) electron beam of the 855 MeV Mainz Microtron MAMI. Transition radiation was observed in the energy range from 2 to 15 keV with a LN2-cooled pin photodiode. A good energy resolution of 0.8 keV and angular resolution of 0.15 mrad was achieved simultaneously allowing for the first time to quantitatively study the interference pattern. Good agreement with theoretical calculations is found. Prospects to exploit transition radiation in the x-ray region from a low e…

PhysicsNuclear and High Energy PhysicsRange (particle radiation)business.industryX-rayRadiationElectromagnetic radiationOpticsTransition radiationCathode rayPhysics::Accelerator PhysicsBeam emittancebusinessMicrotronZeitschrift f�r Physik A Hadrons and Nuclei
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Steering of a Sub-GeV electron beam through planar channeling enhanced by rechanneling

2014

We report the observation of efficient steering of a 855 MeV electron beam at MAMI (MAinzer MIkrotron) facilities by means of planar channeling and volume reflection in a bent silicon crystal. A $30.5\text{ }\text{ }\ensuremath{\mu}\mathrm{m}$ thick plate of (211) oriented Si was bent to cause quasimosaic deformation of the (111) crystallographic planes, which were used for coherent interaction with the electron beam. The experimental results are analogous to those recorded some years ago at energy higher than 100 GeV, which is the only comparable study to date. Monte Carlo simulations demonstrated that rechanneling plays a considerable role in a particle's dynamics and hinders the spoiling…

electron beamEnergy rangesPlanar channelingBent molecular geometryGeneral Physics and AstronomyExtractionCrystallographic planeElectronX-ray sourcesCoherent interactionchanneling; electron beam; beam steerigbeam steerigMonocrystalline siliconPlanarNegative particlesA-particlesVolume reflectionCollimationPhysicsRange (particle radiation)Silicon crystalchannelingNegative particles; Bent crystals; Volume reflection; Deflection; Extraction; Collimation; A-particles; Coherent interaction; Crystallographic plane; Energy ranges; Planar channeling; Silicon crystal; X-ray sourcesReflection (mathematics)Cathode rayPhysics::Accelerator PhysicsAtomic physicsDeflectionBent crystalsEnergy (signal processing)
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SHIPTRAP—a capture and storage facility for heavy radionuclides at GSI

2002

Abstract SHIPTRAP will be an ion-trap facility for heavy radionuclides delivered from SHIP. Ion traps are a perfect instrument for precision measurements since the ions can be cooled to an extremely small phase space and can be stored for a very long time. In addition one can achieve very high purity by removing contaminant ions. SHIPTRAP will extend the possibilities of measurements in traps to transuranium nuclides and provide cooled and isobarically pure ion bunches.

Nuclear physicsPhysicsNuclear and High Energy PhysicsRadionuclideBunchesPhysics::Plasma PhysicsPhysics::Atomic PhysicsNuclideNuclear ExperimentComputer Science::DatabasesTransuranium elementIonNuclear Physics A
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Innovative remotely-controlled bending device for thin silicon and germanium crystals

2020

Steering of negatively charged particle beams below 1 GeV has demonstrated to be possible with thin bent silicon and germanium crystals. A newly designed mechanical holder was used for bending crystals, since it allows a remotely-controlled adjustment of crystal bending and compensation of unwanted torsion. Bent crystals were installed and tested at the MAMI Mainz MIcrotron to achieve steering of 0.855-GeV electrons at different bending radii. We report the description and characterization of the innovative bending device developed at INFN Laboratori Nazionali di Legnaro (LNL).

Physics - Instrumentation and DetectorsMaterials scienceAccelerator ApplicationsSiliconBeam OpticsNegatively charged particleAccelerator Applications; Beam Optics; Instrumentation for particle accelerators and storage rings - high energy (linear accelerators synchrotrons); Instrumentation for particle accelerators and storage rings - lowenergy (linear accelerators cyclotrons electrostatic accelerators); Instrumentation; Mathematical PhysicsBent molecular geometryFOS: Physical scienceschemistry.chemical_elementGermaniumElectron01 natural sciencesInstrumentation for particle accelerators and storage rings - lowenergy (linear accelerators cyclotrons electrostatic accelerators)Instrumentation for particle accelerators and storage rings - high energy (linear accelerators synchrotrons)NOCrystal0103 physical sciencesNuclear Experiment010306 general physicsInstrumentationMicrotronMathematical Physics010308 nuclear & particles physicsbusiness.industryTorsion (mechanics)Instrumentation and Detectors (physics.ins-det)chemistryPhysics::Accelerator PhysicsOptoelectronicsbusinessJournal of Instrumentation
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Novel digital K-edge imaging system with transition radiation from an 855-MeV electron beam

2001

A novel K-edge imaging method has been developed at the Mainz Microtron MAMI aiming at a very efficient use of the transition radiation (TR) flux generated by the external 855-MeV electron beam in a foil stack. A fan-like quasi-monochromatic hard X-ray beam is produced from the /spl plusmn/1-mrad-wide TR cone with a highly oriented pyrolytic graphite (HOPG) crystal. The absorption of the object in front of a 30 mm/spl times/10 mm pn charge-coupled device (pn-CCD) photon detector is measured at every pixel by a broad-band energy scan around the K-absorption edge. This is accomplished by a synchronous variation of the lateral crystal position and the electron beam direction which defines also…

PhysicsNuclear and High Energy Physicsbusiness.industryDetectorchemistry.chemical_elementImaging phantomXenonOpticsNuclear Energy and EngineeringTransition radiationK-edgechemistryHighly oriented pyrolytic graphiteCathode rayElectrical and Electronic EngineeringbusinessMicrotronIEEE Transactions on Nuclear Science
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Channeling experiments with sub-GeV electrons in flat silicon single crystals

2015

Abstract Various planar channeling experiments, performed at the Mainz Microtron MAMI with electrons at silicon single crystals, have been reanalyzed. Two types of signals have been employed. The low energy loss signal originates from emission of channeling radiation in the energy domain between 0.4 and 9 MeV while the high energy loss signal from electrons which have lost about 50% of their primary energy by emission of bremsstrahlung photons. The (1 1 0) planar channeling data, taken at a beam energy of 855 MeV with the former signal, can well be described on the basis of the solution of the classical Fokker–Planck equation. The measurements with the latter signal at beam energies between…

PhysicsNuclear and High Energy PhysicsPhotonSiliconBremsstrahlungchemistry.chemical_elementElectronRadiationCrystalchemistryAtomic physicsNuclear ExperimentInstrumentationMicrotronBeam (structure)Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
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Isotope shift and hyperfine structure measurements at the242f Am fission isomer

1996

Istope shift and hyperfine structure measurements have been performed for the242fAm fission isomer with target production rates of only a few per second. The method is based on resonance ionization spectroscopy (RIS) in a buffer gas cell with radioactive decay detection of the ionization process (RADRIS). A relative isotope shift ratioX exp=IS242f,241/ IS243,241=41.7±0.9 has been measured for the 500.02 nm transition corresponding to a nuclear parameter Λ242f,241=5.4±0.3 fm2. The analysis of the quadrupole moment based on the deformed Fermi-model of the nuclear charge distribution including second order corrections results inQ 20=38.2 ±1.4( −0.8 +0.4 )model eb. The measurement of the hyperf…

Nuclear and High Energy PhysicsIsotopeFissionChemistryCondensed Matter PhysicsAtomic and Molecular Physics and OpticsEffective nuclear chargeIsomeric shiftIsotopic shiftIonizationPhysical and Theoretical ChemistryAtomic physicsHyperfine structureRadioactive decayHyperfine Interactions
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Status of the SHIPTRAP Project: A Capture and Storage Facility for Heavy Radionuclides from SHIP

2001

The ion trap facility SHIPTRAP is being set up to deliver very clean and cool beams of singly-charged recoil ions produced at the SHIP velocity filter at GSI Darmstadt. SHIPTRAP consists of a gas cell for stopping and thermalizing high-energy recoil ions from SHIP, an rf ion guide for extraction of the ions from the gas cell, a linear rf trap for accumulation and bunching of the ions, and a Penning trap for isobaric purification. The progress in testing the rf ion guide is reported. A transmission of about 93(5)% was achieved.

Trap (computing)Nuclear physicsRadionuclideRecoilPhysics::Plasma PhysicsChemistryBuffer gasPhysics::Accelerator PhysicsPhysics::Atomic PhysicsIon trapNuclear ExperimentPenning trapIon
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Investigation of the Electromagnetic Radiation Emitted by Sub-GeV Electrons in a Bent Crystal.

2015

The radiation emitted by 855 MeV electrons via planar channeling and volume reflection in a $30.5\text{\ensuremath{-}}\ensuremath{\mu}\mathrm{m}$-thick bent Si crystal has been investigated at the MAMI (Mainzer Mikrotron) accelerator. The spectral intensity was much more intense than for an equivalent amorphous material, and peaked in the MeV range in the case of channeling radiation. Differently from a straight crystal, also for an incidence angle larger than the Lindhard angle, the spectral intensity remains nearly as high as for channeling. This is due to volume reflection, for which the intensity remains high at a large incidence angle over the whole angular acceptance, which is equal t…

SILICON-CRYSTALSIncoherent scatterGeneral Physics and AstronomyMICROTRON MAMIElectronRadiationMAMI01 natural sciencesElectromagnetic radiationbremsstrahlungNOMAINZPhysics and Astronomy (all)0103 physical sciencescharged particles010306 general physicsRadiant intensityPhysics010308 nuclear & particles physicsScatteringCOHERENT BREMSSTRAHLUNGvolume reflectionSINGLE-CRYSTALcharged particles volume reflection bremsstrahlung performance MAMICHARGED-PARTICLESReflection (physics)Atomic physicsCHARGED-PARTICLES; VOLUME REFLECTION; COHERENT BREMSSTRAHLUNG; SILICON-CRYSTALS; SINGLE-CRYSTAL; MICROTRON MAMI; MAINZIntensity (heat transfer)performancePhysical review letters
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Observation of optical Smith-Purcell radiation at an electron beam energy of 855 MeV.

2002

Smith-Purcell radiation, generated when a beam of charged particles passes close to the surface of a diffraction grating, has been studied in the visible spectral range at wavelengths of 360 and 546 nm with the low emittance 855 MeV electron beam of the Mainz Microtron MAMI. The beam focused to a spot size of $4 \ensuremath{\mu}\mathrm{m}$ (full width at half maximum) passed over optical diffraction gratings of echelle profiles with blaze angles of $0.8\ifmmode^\circ\else\textdegree\fi{}, 17.27\ifmmode^\circ\else\textdegree\fi{},$ and $41.12\ifmmode^\circ\else\textdegree\fi{}$ and grating periods of 0.833 and $9.09 \ensuremath{\mu}\mathrm{m}.$ Taking advantage of the specific emission chara…

DiffractionPhysicsbusiness.industryPhysics::OpticsSynchrotron radiationGratingUndulatorlaw.inventionOpticsTransition radiationlawBlazed gratingPhysics::Accelerator PhysicsAtomic physicsbusinessEnergy (signal processing)Intensity (heat transfer)Physical review. E, Statistical, nonlinear, and soft matter physics
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Impact of buffer gas quenching on the $^1S_0$ $\to$ $^1P_1$ ground-state atomic transition in nobelium

2017

International audience; Using the sensitive Radiation Detected Resonance Ionization Spectroscopy (RADRIS) techniquean optical transition in neutral nobelium (No, Z = 102) was identified. A remnant signal when delaying the ionizing laser indicated the influence of a strong buffer gas induced de-excitation of the optically populated level. A subsequent investigation of the chemical homologue, ytterbium (Yb, Z = 70), enabled a detailed study of the atomic levels involved in this process, leading to the development of a rate equation model. This paves the way for characterizing resonance ionization spectroscopy (RIS) schemes used in the studyof nobelium and beyond, where atomic properties are c…

YtterbiumQuenching (fluorescence)Materials scienceBuffer gaschemistry.chemical_elementRate equation[PHYS.NEXP]Physics [physics]/Nuclear Experiment [nucl-ex]01 natural sciencesAtomic and Molecular Physics and OpticsSpectral line010305 fluids & plasmaschemistry0103 physical sciencesAtomic Physicsddc:530NobeliumPhysics::Atomic PhysicsAtomic physics010306 general physicsGround stateSpectroscopy
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How narrow is the linewidth of parametric X-ray radiation?

1997

Parametric x-ray or quasi-Cherenkov radiation is produced by the passage of an electron through a crystal. A critical absorber technique has been employed to investigate its linewidth. Experiments have been performed with the 855MeV electron beam from the Mainz Microtron MAMI. Thin absorber foils were mounted in front of a CCD camera serving as a position sensitive photon detector. Upper limits of the linewidth of 1.2 and 3.5eV were determined for the (111) and (022) reflections of silicon at photon energies of 4966 and 8332eV. These limits originate from geometrical line broadening effects that can be optimized to reach the ultimate limit given by the finite length of the wave train. {copy…

PhysicsPhotonbusiness.industryGeneral Physics and AstronomyElectronRadiationCrystalLaser linewidthOpticsCathode rayAtomic physicsbusinessMicrotronCherenkov radiation
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First observation of a resonance ionization signal on242mAm fission isomers

1992

The feasibility of a hyperfine spectroscopy on242mAm fission isomers has been demonstrated at the low target production rate of 10/s. The experimental method employed is based on resonance ionization spectroscopy in a buffer gas cell with detection of the ionization process by means of the fission decay of the isomers. The resonance ionization has been performed in two steps, utilizing an excimer dye laser combination with a repetition rate of 300 Hz. The first resonant step proceeds through theJ=7/2 term at 21440.35 cm−1, which has been excited with the tuncable dye laser beam of a wavelength of 466.28 nm, the second non-resonant step is achieved with the 351 nm radiation of the excimer la…

Nuclear and High Energy PhysicsDye laserExcimer laserChemistrymedicine.medical_treatmentAnalytical chemistryPhysics::OpticsResonancePhotoionizationCondensed Matter PhysicsAtomic and Molecular Physics and OpticsAtmospheric-pressure laser ionizationIonizationPhysics::Atomic and Molecular ClustersmedicinePhysics::Atomic PhysicsPhysical and Theoretical ChemistryAtomic physicsSpectroscopyHyperfine structureHyperfine Interactions
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Transition radiation in the x-ray region from a low emittance 855 MeV electron beam

1997

A quasi-monochromatic hard x-ray beam with a photon energy of 33 keV has been produced from transition radiation (TR) at the Mainz Microtron MAMI. The radiator was a stack of 30 polyimide foils of 25 μm thickness and 75 μm separation and the monochromator a highly-oriented pyrolytic graphite crystal. The intrinsic bandwidth was measured with a critical absorption technique to be 100 eV. On the basis of these experiments a photon flux of 4⋅109/mm2s over an illuminated area of 5.7×125 mm2 can be expected from an optimized beryllium radiator at a beam current of 100 μA. At the K-absorption edge of titanium at 5 keV narrow band transition radiation has been observed from a stack of four foils o…

Materials sciencebusiness.industryX-rayPhoton energylaw.inventionOpticsTransition radiationlawCathode rayAtomic physicsbusinessAbsorption (electromagnetic radiation)MicrotronBeam (structure)MonochromatorThe 17th international conference on x-ray and inner-shell processes
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FT-ICR MS studies of ion-molecule reactions of Ru+ and Os+ with oxygen

2005

Abstract The reactions of stored ruthenium and osmium cations with oxygen have been studied in a Fourier transform ion cyclotron resonance (FT-ICR) mass spectrometer. In case of osmium the reaction products OsO+ and OsO 2 + have been observed and corresponding reaction-rate constants have been determined. In addition, there is an unreactive fraction of Os+ ions due to the presence of a slightly endothermic reacting ground state. Only the excited states react with oxygen. For ruthenium no spontaneous reaction with oxygen has been observed unless the cyclotron motion of Ru+ was excited. The results are discussed with respect to a similar investigation in a Penning trap-TOF mass spectrometer […

Analytical chemistrychemistry.chemical_elementCondensed Matter PhysicsMass spectrometryOxygenFourier transform ion cyclotron resonanceHassiumRutheniumIonchemistryExcited stateOsmiumPhysical and Theoretical ChemistryInstrumentationSpectroscopyInternational Journal of Mass Spectrometry
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