Complex chemistry with complex compounds

6533b7d7fe1ef96bd1268402

RESEARCH PRODUCT

Complex chemistry with complex compounds

Sunao Miyashita Sunao Miyashita T. Tomitsuka Yongfeng Wang H. Brand Daiya Kaji M. Murakami N.m. Chiera N.m. Chiera Patrick Steinegger Patrick Steinegger S. Yano Kazuaki Tsukada K. Tanaka Egon Jäger Ch. E. Düllmann Y. Kaneya Alexander Yakushev Birgit Kindler Takayuki Sumita Atsushi Toyoshima Z. Qin Yuichiro Nagame Norbert Wiehl Y. Kudou Mirei Takeyama Y. Wittwer Y. Wittwer Robert Eichler Robert Eichler K. Morimoto S. Yamaki Rugard Dressler N. Sato Jens Volker Kratz F. Fangli H. Haba J. Krier B. Kraus B. Kraus A. Di Nitto Tatsuhiko Sato Julia Even J. Kanaya N. Kurz D. Piguet W. Hartmann Yukiko Komori Yasuo Wakabayashi M. Goetz J. Steiner K. Morita J. Khuyagbaatar I. Usoltsev I. Usoltsev M. Asai Kazuhiro Ooe Andreas Türler Andreas Türler

subject

Physics QC1-999 Transactinide element chemistry.chemical_element Tungsten 010402 general chemistry 010403 inorganic & nuclear chemistry 01 natural sciences 0104 chemical sciences Metal chemistry Group (periodic table)Computational chemistry Molybdenum Chemical physics visual_art Intramolecular force Seaborgium 540 Chemistry Atom visual_art.visual_art_medium 570 Life sciences; biology

description

In recent years gas-phase chemical studies assisted by physical pre-separation allowed for the investigation of fragile single molecular species by gas-phase chromatography. The latest success with the heaviest group 6 transactinide seaborgium is highlighted. The formation of a very volatile hexacarbonyl compound Sg(CO)6 was observed similarly to its lighter homologues molybdenum and tungsten. The interactions of these gaseous carbonyl complex compounds with quartz surfaces were investigated by thermochromatography. Second-generation experiments are under way to investigate the intramolecular bond between the central metal atom of the complexes and the ligands addressing the influence of relativistic effects in the heaviest compounds. Our contribution comprises some aspects of the ongoing challenging experiments as well as an outlook towards other interesting compounds related to volatile complex compounds in the gas phase.

year	journal	country	edition	language
2016-12-01	EPJ Web of Conferences

https://doi.org/10.1051/epjconf/201613107005

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